摘要:Experimental research on non-critical phase-matching fourth harmonic generation with ADP and DKDP crystals are reported. The characteristics of 2 omega-to-4 omega efficiency as function of incident angle, crystal temperature and input 2 omega intensity have been investigated in detail, and the 2 omega-to-4 omega conversion efficiency has been demonstrated up to 84.1% with ADP crystal and 85.1% with DKDP crystal, respectively. Nevertheless, the spatial non-uniformity of rapid grown DKDP crystal has to be improved while the temperature control uniformity should be upgraded for ADP crystal to realize large aperture high efficiency fourth harmonic generation.