标题：Flexible polydimethylsiloxane/multi-walled carbon nanotubes membranous metacomposites with negative permittivity
作者：Sun, Kai; Xie, Peitao; Wang, Zhongyang; Su, Tongming; Shao, Qian; Ryu, JongEun; Zhang, Xihua; Guo, Jiang; Shankar, Akash; Li, Jianfe 更多 作者机构：[Sun, Kai; Fan, Runhua] Shanghai Maritime Univ, Coll Ocean Sci & Engn, Shanghai 201306, Peoples R China.; [Sun, Kai; Xie, Peitao; Wang, Zhongyang; Z 更多
通讯作者地址：[Fan, RH]Shanghai Maritime Univ, Coll Ocean Sci & Engn, Shanghai 201306, Peoples R China;[Guo, ZH]Univ Tennessee, Dept Chem & Biomol Engn, Integrated 更多
关键词：Flexible metamaterials; Negative permittivity; Metacomposites
摘要：Metacomposites with negative electromagnetic parameters can be promising substitute for periodic metamaterials. In this paper, we devoted to fabricating flexible metacomposite films, which have great potential applications in the field of wearable cloaks, sensing, perfect absorption and stretchable electronic devices. The conductivity and the complex permittivity were investigated in flexible polydimethylsiloxane (PDMS)/multi-walled carbon nanotubes (MWCNTs) membranous nanocomposites, which were fabricated via in-situ polymerization process. With the increase of conductive onedimension carbon nanotubes concentration, there was a percolation transition observed in conduction due to the formation of continuous networks. The dielectric dispersion behavior was also analyzed in the spectra of complex permittivity. It is indicated that the conduction and polarization make a combined effect on the dielectric loss in flexible PDMS/MWCNTs composites. The negative permittivity with a dielectric resonance was obtained, and was attributed to the induced electric dipoles. (C) 2017 Published by Elsevier Ltd.