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III-->II were observed from above three kinds of phase diagrams with increasing the concentration of alcohol, It was observed from the Winsor phase diagram that the phase types, the phase volumes and the concentrations of alcohol at the start point and end point of the Winsor microemulsion formation change with the increase of the concentration of alcohol. From the delta-gamma fishlike phase diagram, some important parameters were calculated, such as the mass fraction of 1-butanol in the hydrophile-lipophile balanced interfacial layer, A(s), the coordinates of the start point and the end point of the Winsor microemulsion formation, and the solubilities of APG and 1-butanol in n-octane phase. The modified epsilon-beta fishlike phase diagram was presented for the first time by us. With the epsilon-beta fishlike phase diagram, the above experimental phenomena were observed and the physico-chemical parameters were calculated precisely. The epsilon-beta fishlike phase diagram has some advantages over the Winsor and delta-gamma fishlike phase diagrams in visual observations of the phase changes, and calculation of the related physico-chemical parameters. [author_in] => [Chai, J.-L] Key Laboratory for Colloid and Interface Chemistry, Ministry of Education, Shandong University, Jinan 250100, China, Department of Chemistry, Shandong Normal University, Jinan 250014, China@@@[ Li, D.-X] Key Laboratory for Colloid and Interface Chemistry, Ministry of Education, Shandong University, Jinan 250100, China@@@[ Li, G.-Z] Key Laboratory for Colloid and Interface Chemistry, Ministry of Education, Shandong University, Jinan 250100, China@@@[ Liang, F.-Z] Department of Chemistry, Shandong Normal University, Jinan 250014, China@@@[ Zhang, G.-Y] Key Laboratory for Colloid and Interface Chemistry, Ministry of Education, Shandong University, Jinan 250100, China@@@[ Xia, R] Beijing Municipal Institute of Drug Controls, Beijing 100035, China [publication_type] => J [begin_page] => 47 [author_en] => Chai, JL; Li, DX; Li, GZ; Liang, FZ; Zhang, GY; Xia, R [volume] => 62 [get_data] => 2018-08-29 [publisher] => SCIENCE CHINA PRESS [keyword_en] => middle-phase microemulsion; fishlike phase diagram; alkyl polyglucoside;; solubilization [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [keyword_plu] => GLYCEROL ETHER; BEHAVIOR; SYSTEMS; SURFACTANTS [publication_iso] => Acta Chim. Sin. 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[keyword_cn] => 树枝状化合物;液晶;光电信息功能材料;量子产率;反-顺光异构化;光回复异构;反/顺异构组分化;热回复异构;活化能 [article_id] => 597892,239571,491858,664148,330995,68716 [clc] => Q516 [author_jg] => [张其震,刘建强,殷晓颖,张静智]山东大学化学化工学院,山东大学化学化工学院物理与微电子学院,山东大学化学化工学院,山东大学化学化工学院 济南 250100, 济南 250100, 济南 250100, 济南 250100 [format_title_cn_publication_cn_pub_year] => c18ac09dab157f52dcba8c7a9e7e1443324757932 [hints] => 18 [issue] => 7 [sys_level_num] => 2_3 [sys_jg_type] => 11,3,5 [format_issn_issue_page_pub_year] => d752225e0173ccee25f836f85dbd62e6-277651012 [source_type] => 351 [pub_year] => 2003 [pub_date] => JUL [pages] => 6 [from_id] => 76,75,73,80,85,78 [author_cn] => 张其震,刘建强,殷晓颖,张静智 [issn] => 0567-7351 [uri] => http://kns.cnki.net/kns/detail/detail.aspx?FileName=HXXB200307025&DbName=CJFQ2003 [publication_cn] => 化学学报 [title_cn] => 一代树状碳硅烷液晶的光化学研究——端基含12个4-丁氧基偶氮苯介晶基元 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => c2b6637872211b85f7a63df52b38e8b945432130 [page] => 1108-1113 [hb_type] => 2 [article_dt] => Article [hb_batch] => title_cn_publication_cn_pub_year_2_3 [format_title_en] => 13d15c6ce0b42526df172c769b9f7deb1508578682 [format_title] => 845ed12b002349b8631ae8d2afc096ef758132574 [hx_id] => 2377,2378,2371 [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [format_publication_en] => 169b60c7845c9e5f36906950b18f11111348184734 [jl_publication_cn] => 化学学报 [jl_article_dt] => 期刊论文 [jl_keyword_cn] => 光电信息功能材料,热回复异构,活化能,量子产率,反顺异构组分化,光回复异构,液晶,反顺光异构化,树枝状化合物 [jl_clc] => q516 [author_in] => [Zhang, Q.-Z] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China@@@[ Liu, J.-Q] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China, School of Physics and Microelectronics, Shandong University, Jinan 250100, China@@@[ Yin, X.-Y] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China@@@[ Zhang, J.-Z] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China [company_id] => 43,35,133,0,5,169 [sys_subject_sort] => 0,0,0,0,0 [college_parent_id] => 133,5,43,35,169 [company_test] => Array,Array,Array,Array,Array [author_id] => [author_test] => Array ( ) [sys_author_id_arr] => [jl_publication_cn_publication_en] => 化学学报 [jl_keyword_cn_keyword_en] => 液晶,树枝状化合物,活化能,光回复异构,热回复异构,量子产率,反顺光异构化,光电信息功能材料,反顺异构组分化 [cite_wos] => 11 [publication_en] => ACTA CHIMICA SINICA [fund_No] => 国家自然科学基金(Nos. 29874020, 59573029); 山东省自然科学基金(No. Y95B0720); 中国科学院高分子物理重点实验室(长春应用化学研究所)资助项目 [check_3Y] => 1 [language] => Chinese [delivery_No] => 715TM [cauthor_ad] => [Zhang, QZ]Shandong Univ, Sch Chem & Chem Engn, Jinan 250100, Peoples R China. [author_fn] => Zhang, QZ; Liu, JQ; Yin, XY; Zhang, JZ [reference] => Archut A, 1998, Am. Chem. Soc, V120, P12187@@@IKEDA T, 1995, SCIENCE, V268, P1873, DOI 10.1126/science.268.5219.1873@@@Junge DM, 1999, J AM CHEM SOC, V121, P4912, DOI 10.1021/ja990387+@@@Lorenz K, 1996, ADV MATER, V8, P414, DOI 10.1002/adma.19960080509@@@Nagasaki T, 1997, CHEM LETT, P717, DOI 10.1246/cl.1997.717@@@PERCEC V, 1995, J AM CHEM SOC, V117, P11441, DOI 10.1021/ja00151a008@@@Ponomarenko SA, 1996, LIQ CRYST, V21, P1, DOI 10.1080/02678299608033789@@@[张其震 Zhang Qizhen], 2003, [化学学报, Acta Chemical Sinica], V61, P619@@@[张其震 Zhang Qizhen], 2003, [化学学报, Acta Chemical Sinica], V61, P416@@@[张其震 Zhang Qizhen], 2002, [化学学报, Acta Chemical Sinica], V60, P2232@@@张其震, 1998, 高等学校化学学报, V19, P1175@@@张其震, 1997, 高等学校化学学报, V18, P158@@@张静智, 1997, 化学学报, V55, P930@@@张其震, 1996, 高分子学报, P121@@@张其震, 1998, 高等学校化学学报.J, V9, P827@@@张其震, 2000, 功能高分子材料.第11章 [cite_wanfang] => 20 [cauthor] => Zhang, QZ(qzzhang@sdu.edu.cn) [format_title_en_issn_pub_year] => 10b075ae498dedd5458421154f7a484e-637982662 [datebase] => Scopus [format_scopus_No] => 422ae9e09c743448639fa4f02177c67c-610934877 [publication_29] => ACTA CHIM SINICA [end_page] => 1113 [abstract_en] => The quantum yield, trans/cis photoisomerization, photo back-isomerization, trans/cis isomer ratio, thermal back-isomerization activation energy of a new carbosilane liquid crystalline (LC) dendrimer of the first generation (D1) containing twelve 4-butoxyazobenzene mesogen in its periphery and azobenzene unit compound M5 in CHCl3, THF, DMF, EtOH and C6H6 are described. Photochromic rate constant of D1 and M5 are 10(-1) s(-1), but that of photochromic LC polysiloxanes containing the same azobenzene moieties is 10(-8) s(-1) thus the photoresponsive rate of LC dendrimer D1 is 10(7) times larger than that of the latter. [publication_type] => J [begin_page] => 1108 [author_en] => Zhang, QZ; Liu, JQ; Yin, XY; Zhang, JZ [format_cscd_No] => a683658c518b49748c7282b0f35cef0c513362855 [volume] => 61 [publisher] => SCIENCE CHINA PRESS [get_data] => 2018-08-29 [keyword_en] => dendrimer; liquid crystal; photo-electro informational functional; material; quantum yield; trans/cis photoisomerization; photo; back-isomerization; trans/cis isomer ratio; thermal back-isomerization;; activation energy [publication_iso] => Acta Chim. Sin. [format_title_en_publication_en_pub_year] => 12bbbb9a92a516e3bc667dbbf9346732-1858133464 [cite_scopus] => 11 [publisher_city] => BEIJING [cite_cscd] => 10 [publication_info] => 0567-7351(2003)61:7<1108:YDSZTG>2.0.TX;2-N [email_c] => qzzhang@sdu.edu.cn [email] => qzzhang@sdu.edu.cn [reference_No] => 16 [cite_awos] => 12 [cscd_No] => CSCD:1174257 [wos_No] => WOS:000184988400026 [format_wos_No] => 6066d39809f3d47fb1420d1ab73aa683-1747501829 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [check_180] => 0 [publisher_ad] => 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA [standard_in] => School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China; School of Physics and Microelectronics, Shandong University, Jinan 250100, China [scopus_No] => 2-s2.0-20444453950 [title_en] => Study on photochemistry of carbosilane liquid crystalline dendrimer of the first generation - Containing twelve 4-butoxyazobenzene mesogenic groups in its periphery [jl_language] => chinese [jl_publication_en] => actachimicasinica [sys_author_jg_last_arr] => 济南250100 [jl_company_test] => unameuu5316u5b66u4e0eu5316u5de5u5b66u9662,unameuu5faeu7535u5b50u5b66u9662,uorgidu5,uparentidu35,uparentidu43,unameuu7269u7406u5b66u9662,uircu0,uorgidu43,ulevelu1,uorgidu35,uparentidu5 [jl_country] => 中国 [jl_keyword_en] => ,photoelectroinformationalfunctional,photo,material,backisomerization,thermalbackisomerization,transcisphotoisomerization,transcisisomerratio,liquidcrystal,activationenergy,dendrimer,quantumyield [sys_author_in_last_arr] => china [jl_publisher] => sciencechinapress [sys_author_id] => [id] => MA5HvmUBFjIhTVEbZSTq [tags] => 0 ) [15] => Array ( [batch2] => 1,2,6 [uri] => https://www.scopus.com/inward/record.uri?eid=2-s2.0-33750439156&partnerID=40&md5=2f93640f6aaf8a2eaf206d877b9856a8 [tag] => 0 [abstract_cn] => 用自组装技术在铜电极表面上制备了纯烯丙基硫脲自组装膜 ,并以十二烷基硫醇进一步修饰得到混合自组装膜 .最后 ,将混合膜覆盖的铜电极浸入NaCl溶液中 ,进行交流电处理 .电化学交流阻抗谱和极化曲线测定表明 ,经过交流电处理后 ,在 0 .5mol·dm- 3NaCl溶液中 ,电荷传递电阻增大 ,腐蚀电流密度下降 ,膜的最大覆盖度为 98.6% ,对金属铜腐蚀的缓蚀效率为 98.5 % .而且 ,不论交流电处理与否 ,混合自组装膜在较宽的电极电位范围内均表现出很强的稳定性 [keyword_cn] => 自组装;;电化学交流阻抗;;交流电处理;;缓蚀效率 [fund_No] => 国家自然科学基金(No.20173033); 国家重点基础研究专项经费(No.G19990650)资助项目 [article_id] => 239574,26628,581877,491802,663281,331608 [clc] => O657.3 [author_jg] => [王春涛] 山东大学化学与化工学院, 济南, 山东 250100, 中国.@@@[陈慎豪] 山东大学化学与化工学院, 济南, 山东 250100, 中国.@@@[赵世勇] 山东大学化学与化工学院, 济南, 山东 250100, 中国.@@@[李德刚] 山东大学化学与化工学院, 济南, 山东 250100, 中国 [format_title_cn_publication_cn_pub_year] => 4082d1972ebf7559942ffbe91d38d2ed-764640997 [hints] => 10 [issue] => 2 [author_first] => 王春涛 [sys_level_num] => 2_3 [sys_jg_type] => 3,5 [format_issn_issue_page_pub_year] => d28b087a20aed739c97d6e9ea62e8334141953952 [source_type] => 351 [pub_year] => 2003 [pub_date] => FEB [pages] => 5 [from_id] => 76,75,73,80,78,85 [author_cn] => 王春涛;陈慎豪;赵世勇;李德刚 [issn] => 0567-7351 [batch] => 3249,3250,3252,3254,3243,3241 [publication_cn] => 化学学报 [title_cn] => 烯丙基硫脲和十二烷基硫醇对铜的缓蚀作用 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => e789edab9d93e455fcd7f4da14d9ca14-1441745287 [page] => 151-155 [hb_type] => 2 [article_dt] => Article [hb_batch] => title_cn_publication_cn_pub_year_2_3 [publication_en] => ACTA CHIMICA SINICA [cite_wos] => 10 [check_3Y] => 4 [language] => Chinese [delivery_No] => 648VU [format_title] => 44258f7c814e336542632261bf46d5b91006423409 [cauthor_ad] => [Chen, SH]Shandong Univ, Sch Chem & Chem Engn, Jinan 250100, Peoples R China. [author_fn] => Wang, CT; Chen, SH; Zhao, SY; Li, DG [reference] => BARCIA OE, 1993, J ELECTROCHEM SOC, V140, P2825, DOI 10.1149/1.2220917@@@Brown G M, 1995, J electroanal Chem, V38, P161@@@Cui XL, 2000, COLLOID SURFACE A, V175, P141, DOI@@@10.1016/S0927-7757(00)00528-8@@@@@@Deslouis C, 1988, J Appl Electrochem, V16, P374@@@Diao P, 1999, J ELECTROANAL CHEM, V464, P61, DOI@@@10.1016/S0022-0728(98)00470-7@@@Feng Y, 1996, CORROS SCI, V38, P369, DOI 10.1016/0010-938X(96)00110-2@@@Feng YQ, 1997, J ELECTROCHEM SOC, V144, P55, DOI 10.1149/1.1837365@@@Folquer ME, 2002, CORROSION, V58, P240, DOI 10.5006/1.3279875@@@@@@Itoh M, 1995, Electrochem Soc, V142, P1839@@@Jennings GK, 1998, LANGMUIR, V14, P6130, DOI 10.1021/la980333y@@@Kim T, 1997, J AM CHEM SOC, V119, P189, DOI 10.1021/ja9617956@@@@@@LAIBINIS PE, 1992, J AM CHEM SOC, V114, P9022, DOI 10.1021/ja00049a038@@@Lee H P, 1996, Electrochem Soc, V133, P2035@@@LOO BH, 1982, CHEM PHYS LETT, V89, P346, DOI@@@10.1016/0009-2614(82)83513-6@@@@@@Ma H, 2002, J APPL ELECTROCHEM, V32, P65, DOI 10.1023/A:1014242112512@@@Matsumoto F, 1999, LANGMUIR, V15, P857, DOI 10.1021/la980919k@@@NAHIR TM, 1994, ELECTROCHIM ACTA, V39, P2347, DOI@@@10.1016/0013-4686(94)00209-6@@@@@@SABATANI E, 1993, LANGMUIR, V9, P2974, DOI 10.1021/la00035a040@@@SCHONENBERGER C, 1994, LANGMUIR, V10, P611, DOI 10.1021/la00015a001@@@TIAN ZQ, 1990, ELECTROCHIM ACTA, V35, P879, DOI@@@10.1016/0013-4686(90)90084-D@@@@@@Wang J, 2000, ANAL SCI, V16, P457, DOI 10.2116/analsci.16.457@@@Yamamoto Y, 1993, Electrochem Soc, V140, P436 [publication_29] => ACTA CHIM SINICA [end_page] => 155 [abstract_en] => Self-assembled monolayer of allylthiourea (AT) was first formed on copper surface. 1-Dodecanethiol (DT) was then self-assembled on the surface for subsequent modification: Finally, AC voltage was loaded on copper covered with the mixed film for further improvement. After these processes, an effective inhibition film was obtained as indicated by the high charge-transfer resistance shown in electrochemical impedance spectroscopy and low corrosion current density in polarization curves. The maximum coverage and inhibition efficiency for copper corrosion was 98.6% and 98.5%, respectively. The mixed film was stable in a wide range of potential before and after AC voltage treatment. [author_in] => [Wang, C.-T] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China@@@[ Chen, S.-H] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China, State Key Laboratory for Corrosion and Protection, Shenyang 110015, China@@@[ Zhao, S.-Y] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China@@@[ Li, D.-G] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China [publication_type] => J [begin_page] => 151 [author_en] => Wang, CT; Chen, SH; Zhao, SY; Li, DG [volume] => 61 [get_data] => 2018-08-29 [publisher] => SCIENCE CHINA PRESS [keyword_en] => self-assembly; electrochemical impedance spectroscopy; AC treatment;; inhibition efficiency [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [keyword_plu] => SELF-ASSEMBLED MONOLAYERS; IMPEDANCE SPECTROSCOPY; ACID-SOLUTION; GOLD; PROTECTION; ALKANETHIOLS; ELECTRODE; THIOUREA; ELECTRODISSOLUTION; MECHANISMS [publication_iso] => Acta Chim. Sin. 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[keyword_cn] => SE相液晶;胆甾相液晶;一代树状化合物;4-硝基偶氮苯;碳硅烷 [article_id] => 661939,491947,239576,331008,105806,539408 [clc] => O621 [author_jg] => [张其震] 山东大学化学化工学院, 济南, 山东 250100, 中国.@@@[盛昕] 山东大学化学化工学院, 济南, 山东 250100, 中国.@@@[殷晓颖] 山东大学化学化工学院, 济南, 山东 250100, 中国.@@@[季怡萍] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国.@@@[李光] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国.@@@[赵晓光] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国 [format_title_cn_publication_cn_pub_year] => 8170dfac23db0c4ed46e5db92b935c16 [hints] => 10 [issue] => 9 [sys_level_num] => 2_3 [sys_jg_type] => 11,5 [format_issn_issue_page_pub_year] => c1db1e67b6543d484c32d48aa06c3e5f [source_type] => 351 [pub_year] => 2003 [pub_date] => SEP [pages] => 6 [from_id] => 76,75,73,80,78,85 [author_cn] => 张其震,盛昕,殷晓颖,季怡萍,李光,赵晓光 [issn] => 0567-7351 [uri] => https://www.scopus.com/inward/record.uri?eid=2-s2.0-33750478392&partnerID=40&md5=15bb4c1b81de8c4567709cc21599978d [publication_cn] => 化学学报 [title_cn] => 一代树状碳硅烷液晶研究——端基含12个4-硝基偶氮苯介晶基元 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => e9121686c8acc7935fee06bf45efc226 [page] => 1478-1483 [hb_type] => 2 [article_dt] => Article [hb_batch] => title_cn_publication_cn_pub_year_2_3 [publication_en] => ACTA CHIMICA SINICA [cite_wos] => 10 [fund_No] => 国家自然科学基金(Nos.29874020,59573029); 中国科学院高分子物理重点实验室基金(中国科学院长春应用化学研究所Nos.R 149833C,R159633Q,R159833C)资助项目; 山东省自然科学基金(No.Y95B0720) [check_3Y] => 1 [language] => Chinese [delivery_No] => 765AX [format_title] => 18dc671fa82aae1df82250ae3dad3429-2143997399 [cauthor_ad] => [Zhang, QZ]Shandong Univ, Sch Chem & Chem Engn, Jinan 250100, Peoples R China. [author_fn] => Zhang, QZ; Sheng, X; Yin, XY; Ji, YP; Li, G; Zhao, XG [reference] => Archut A, 1998, J AM CHEM SOC, V120, P12187, DOI 10.1021/ja9822409@@@@@@de Vries A, 1985, Mol. Cryst. Liq. Cryst., V131, P125@@@DEMUS L, 1978, TEXTURES LIQUID CRYS, P55@@@FINKELMAN H, 1991, LIQUID CRYSTALLINITY, P256@@@FISHWICK M, 1970, J ORGANOMET CHEM, V25, P69, DOI@@@10.1016/S0022-328X(00)86206-3@@@@@@FURNISS BS, 1978, VOGELS TXB PRACTICAL, P715@@@GRAY CW, 1984, SMECTIC LIQUID CRYST, P21@@@Hudson SD, 1997, SCIENCE, V278, P449, DOI 10.1126/science.278.5337.449@@@JANGE DM, 1999, J AM CHEM SOC, V121, P4912@@@KANG SK, 1985, SYNTHESIS-STUTTGART, P1161@@@Karstedt B, 1973, US 3775452@@@Nagasaki T, 1997, CHEM LETT, P717, DOI 10.1246/cl.1997.717@@@PERCEC V, 1995, J AM CHEM SOC, V117, P11441, DOI 10.1021/ja00151a008@@@Pesak DJ, 1997, ANGEW CHEM INT EDIT, V36, P1636, DOI@@@10.1002/anie.199716361@@@@@@Ponomarenko SA, 1996, LIQ CRYST, V21, P1, DOI 10.1080/02678299608033789@@@[唐新德 Tang XinDe], 2003, [有机化学, Chinese Journal of Organic Chemistry],@@@V23, P238@@@van der Made A W, 1992, J. Chem. Soc., Chem. Commun, P1400@@@[张其震 Zhang Qizhen], 2003, [化学学报, Acta Chemical Sinica], V61, P619@@@[张其震 Zhang Qizhen], 2003, [化学学报, Acta Chemical Sinica], V61, P1108@@@[张其震 Zhang Qizhen], 2003, [化学学报, Acta Chemical Sinica], V61, P416@@@[张其震 Zhang Qizhen], 2002, [化学学报, Acta Chemical Sinica], V60, P2232@@@张其震, 1998, 高等学校化学学报, V19, P1175@@@张其震, 1998, 高等学校化学学报, V19, P827@@@张其震, 1997, 高等学校化学学报, V18, P158@@@周其凤, 1994, 液晶高分子@@@张其震, 2000, 功能高分子材料 [publication_29] => ACTA CHIM SINICA [end_page] => 1483 [abstract_en] => The divergent synthesis of a new carbosilane liquid crystalline (LC) dendrimer of the first generation (D1) is described. Twelve 4-nitroazobenzene are used as mesogenic fragments and attached in its periphery and fourcarbosilane as core. Structure and properties of D1 were characterized by elemental analysis, H-1 NMR, MALDITOF-MS, IR, UV-vis, polarizing optical micrograph, DSC and WAXD. Mesogenic compound NU exhibits nematic and dendrimer D1 reveals cholesteryl and smectic E liquid crystalline state. Phase behavior of D1 in LC state is K70Ch188I185Ch58S(E)48K. [author_in] => [Zhang, Q.-Z] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China@@@[ Sheng, X] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China@@@[ Yin, X.-Y] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China@@@[ Ji, Y.-P] Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China@@@[ Li, G] Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China@@@[ Zhao, X.-G] Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China [publication_type] => J [begin_page] => 1478 [author_en] => Zhang, QZ; Sheng, X; Yin, XY; Ji, YP; Li, G; Zhao, XG [volume] => 61 [get_data] => 2018-08-29 [publisher] => SCIENCE CHINA PRESS [keyword_en] => smectic E liquid crystal; cholesteryl liquid crystal; dendrimer of the; first generation; 4-nitroazobenzene; carbosilane [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [keyword_plu] => MOLECULES [publication_iso] => Acta Chim. Sin. [format_title_en] => 72e6a710dc200fc72d3fa13a072b072f1961440278 [publisher_city] => BEIJING [hx_id] => 2377,2378,2371 [reference_No] => 26 [email] => qzzhang@sdu.edu.cn [cite_awos] => 10 [wos_No] => WOS:000188245700026 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [check_180] => 0 [publisher_ad] => 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA [title_en] => Study on a carbosilane liquid crystalline dendrimer of the first generation - Containing twelve 4-nitroazobenzene mesogen in its periphery [format_publication_en] => 169b60c7845c9e5f36906950b18f11111348184734 [jl_language] => chinese [jl_publication_cn] => 化学学报 [jl_article_dt] => 期刊论文 [jl_publication_en] => actachimicasinica [jl_country] => 中国,纳米比亚,瑞士,印度 [jl_keyword_en] => dendrimerofthe,carbosilane,smecticeliquidcrystal,firstgeneration,cholesterylliquidcrystal,4nitroazobenzene [jl_keyword_cn] => 碳硅烷,se相液晶,一代树状化合物,4硝基偶氮苯,胆甾相液晶 [jl_clc] => o621 [jl_publisher] => sciencechinapress [company_id] => 43,169 [sys_subject_sort] => 0,0 [college_parent_id] => 43,169 [company_test] => Array,Array [author_id] => 21651,25088,21654,25613,25608,25110 [author_test] => Array ( [0] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 5 [name] => 李广 [irtag] => 7 [t_index] => 0 [person_id] => 21654 ) [1] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 1 [name] => 张群姿 [irtag] => 8 [t_index] => 1 [person_id] => 25613 ) [2] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 1 [name] => 张庆竹 [irtag] => 7 [t_index] => 1 [person_id] => 25608 ) [3] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 3 [name] => 尹向勇 [irtag] => 7 [t_index] => 0 [person_id] => 25110 ) [4] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 5 [name] => 李刚 [irtag] => 7 [t_index] => 0 [person_id] => 21651 ) [5] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 3 [name] => 殷向阳 [irtag] => 7 [t_index] => 0 [person_id] => 25088 ) ) [sys_author_id_arr] => [cscd_No] => CSCD:1240527 [jl_publication_cn_publication_en] => 化学学报,actachimicasinica [jl_keyword_cn_keyword_en] => 碳硅烷,胆甾相液晶,4硝基偶氮苯,一代树状化合物,se相液晶,dendrimerofthe,carbosilane,smecticeliquidcrystal,4nitroazobenzene,cholesterylliquidcrystal,firstgeneration [sys_author_id] => [format_cscd_No] => 1a6c961ad307e103e8df8f6f9926c588 [format_title_en_publication_en_pub_year] => 9ad6c9357e51940acf84d2006a097042 [format_wos_No] => 637169992029da2a60fba69bc1ad9797 [format_title_en_issn_pub_year] => 69741bfe6e6e1b16603d457bb97c0f65 [format_scopus_No] => d0da8f3645bfba0c40230695d3bc7d88 [standard_in] => School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China; Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China [cauthor] => Zhang, QZ(qzzhang@sdu.edu.cn) [datebase] => Scopus [cite_scopus] => 8 [sys_priority_field] => 76 [scopus_No] => 2-s2.0-33750478392 [jl_pub_year] => 2003 [jl_author_test] => unameuu5f20u7fa4u59ff,usureu0,unameuu6bb7u5411u9633,unameuu5f20u5e86u7af9,unameuu5c39u5411u52c7,uuindex3,uuindex1,upersonid25110,utindex1,utindex0,uirtag7,upersonid21654,upersonid21651,upersonid25608,upersonid25088,unameuu674eu521a,unameuu674eu5e7f,uuindex5,upersonid25613,uirtag8 [sys_author_jg_last_arr] => 中国 [jl_company_test] => uircu0,unameuu5316u5b66u4e0eu5316u5de5u5b66u9662,uparentidu43,uorgidu43,ulevelu1 [sys_author_in_last_arr] => china [id] => _A9KvmUBFjIhTVEbYgQg [tags] => 0 ) [17] => Array ( [batch2] => 1,2 [batch] => 3250,3241,3254,3252 [tag] => 0 [abstract_cn] => 本文合成了具有隔室构造的Schiff碱配体H_3L(L~(3-)=C_(11)H_(11)N_6OS_2~(3-)),并对其进行了元素分析,IR,~1H NMR和MS等项表征.制备了该配体的分别由醋酸根和吡啶分子协配的两种锌的双核配合物,对后者进行了X射线单晶结构分析.[Zn_2L(OH)(py)_2](Py)_2,P2_1/c,a=0.9195(1),b=2.3334(6),c=1.6111(3)nm,β=93.99(1)°,Z=4.结构用直接法解得,最终的R=0.066.测定的结果表明,两锌原子间存在酚氧和羟基的两μ_2-O-桥,每个五配位的锌均具有四方锥型的配位构型. [keyword_cn] => Schiff碱配体;双核锌配合物;晶体结构 [article_id] => 170606,335581,539395,106122 [clc] => O641.4 [author_jg] => [马长勤,王绪宁,张文兴,于正刚,蒋德华,董士利]山东大学化学院,山东大学化学院,山东大学化学院,山东大学化学院,山东大学化学院,淄博市公安局 济南250100,济南250100,济南250100,济南250100,济南250100,淄博255039 [format_title_cn_publication_cn_pub_year] => d0bfd133d1197a8f0072fe547c29e8791048131311 [hints] => 19 [issue] => 6 [sys_level_num] => 2_3 [sys_jg_type] => 5 [format_issn_issue_page_pub_year] => 541eb4e0ecfe7d2c817d83d9d34432aa-1299104508 [source_type] => 351 [pub_year] => 1996 [pub_date] => 1996-06-20 [pages] => 6 [from_id] => 80,78,73,85 [author_cn] => 马长勤,王绪宁,张文兴,于正刚,蒋德华,董士利 [issn] => 0567-7351 [uri] => http://kns.cnki.net/kns/detail/detail.aspx?FileName=HXXB199606006&DbName=CJFQ1996 [publication_cn] => 化学学报 [title_cn] => 含N,O和S的Schiff碱配体的双核锌配合物的合成与晶体结构 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => 830e4c0795d107904455dd94896af91b-1399008932 [page] => 562-567 [hb_type] => 2 [article_dt] => Article [hb_batch] => title_cn_publication_cn_pub_year_2_3 [format_title_en] => 4cb6957559cd6e825d32254ba816292b-818012582 [format_title] => b42d7eb077b76b7d2178d0e929283e43-286254877 [hx_id] => 2371 [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [format_publication_en] => 169b60c7845c9e5f36906950b18f11111348184734 [jl_publication_cn] => 化学学报 [jl_article_dt] => 期刊论文 [jl_keyword_cn] => schiff碱配体,晶体结构,双核锌配合物 [jl_clc] => o6414 [author_in] => [company_id] => 0,43,169 [sys_subject_sort] => 0,0 [college_parent_id] => 43,169 [company_test] => Array,Array [author_id] => [author_test] => Array ( ) [sys_author_id_arr] => [jl_publication_cn_publication_en] => 化学学报 [jl_keyword_cn_keyword_en] => 晶体结构,双核锌配合物,schiff碱配体 [sys_author_id] => [cite_wos] => 10 [publication_en] => ACTA CHIMICA SINICA [check_3Y] => 0 [language] => Chinese [delivery_No] => UY132 [cauthor_ad] => [Ma, CQ]SHANDONG UNIV,COLL CHEM,JINAN 250100,PEOPLES R CHINA. [author_fn] => Ma, CQ; Wang, XN; Zhang, WX; Yu, ZG; Jiang, DH; Dong, SL [format_title_en_issn_pub_year] => 616f0d6a37643129464f444a89d65e811586679960 [publication_29] => ACTA CHIM SINICA [end_page] => 567 [abstract_en] => A compartmental Schiff base ligand H(3)L(L(3-) = C11H11N6OS23-) has been synthesized and characterized by elemental analyses, H-1 NMR, IR and MS as well as etc.. Its dinuclear zinc complex, which are co-coordinated by acetate radicals and pyridine molecules respectively, have been prepared. For the later the single crystal structure has been determinated by X-ray diffraction. [Zn(2)L(OH)(py)(2)](py)(2), P2(1)/c, a = 0.9195(1), b = 2.3334(6), c = 1.6111(3), beta = 93.99(1)degrees, Z = 4. The structure was solved by direct method. The refinement converges with R = 0.066 and R(w) = 0.070 based on 2028 reflections with I greater than or equal to 3 sigma(I). The results indicate that between two zinc atoms exist two mu(2) - O- bridges formed by a phenolic oxygen atom and a hydroxy group in the lattice, respectively; and every five-coordinate zinc atom possesses a square pyramidal construction. [publication_type] => J [begin_page] => 562 [author_en] => Ma, CQ; Wang, XN; Zhang, WX; Yu, ZG; Jiang, DH; Dong, SL [volume] => 54 [get_data] => 2018-08-29 [publisher] => ACTA CHIMICA SINICA [keyword_plu] => METAL [publication_iso] => Acta Chim. Sin. [format_title_en_publication_en_pub_year] => 6f2ce8815607540212db0ef04639c663-64175109 [publisher_city] => SHANGHAI [cauthor_order] => 1 [reference_No] => 6 [cite_awos] => 10 [wos_No] => WOS:A1996UY13200007 [format_wos_No] => 9a9b5ba9621c953e1101135ffa159b27-811654138 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [cauthor_back] => Ma, CQ [check_180] => 0 [publisher_ad] => SHANGHAI INST ORGANIC CHEM ACADEMIA SINICA 345 LINGLING LU, SHANGHAI,; PEOPLES R CHINA [title_en] => Syntheses and crystal structure of dinuclear zinc complex with Schiff base ligand containing N, O and S dornors [id] => 7w9KvmUBFjIhTVEbYAQa [tags] => 0 ) [18] => Array ( [batch2] => 1,2,6 [batch] => 3249,3250,3241,3254,3243,3252 [tag] => 0 [abstract_cn] => 采用耗散颗粒动力学(DPD)方法在介观层次上模拟了表面活性剂烷基苯磺酸盐在油,水界面的排布行为,考察了分子结构、浓度、盐度、油相等因素对表面活性剂界面密度和界面效率的影响,并探讨了利用表面活性剂复配协同效应提高界面活性的理论机制、分子模拟给出的分子水平的微观信息为强化采油技术中配方筛选和表面活性剂的有效应用提供指导. [keyword_cn] => 耗散颗粒动力学模拟;界面密度;界面效率;烷基苯磺酸盐; [clc] => TE357.46 [author_jg] => [李振泉] 中石化胜利油田地质科学研究院, 东营, 山东 257015, 中国.@@@[曹绪龙] 中石化胜利油田地质科学研究院, 东营, 山东 257015, 中国.@@@[宋新旺] 中石化胜利油田地质科学研究院, 东营, 山东 257015, 中国.@@@[崔晓红] 中石化胜利油田地质科学研究院, 东营, 山东 257015, 中国.@@@[何秀娟] 山东大学化学与化工学院, 胶体与界面教育部重点实验室, 济南, 山东 250100, 中国.@@@[李英] 山东大学化学与化工学院, 胶体与界面教育部重点实验室, 济南, 山东 250100, 中国.@@@[马保民] 山东大学化学与化工学院, 胶体与界面教育部重点实验室, 济南, 山东 250100, 中国 [format_title_cn_publication_cn_pub_year] => 3bd82ec1f23ceb55ae8fe9bb03391eaf-337526265 [from_id] => 76,75,73,80,78,85 [issue] => 24 [sys_level_num] => 2_1 [sys_jg_type] => 11,10,5 [source_type] => 351 [pub_year] => 2007 [article_id] => 620591,323864,483511,33887,238487,662743 [pages] => 6 [hints] => 12 [author_cn] => 李振泉[2];何秀娟[1];李英[1];马保民[1];曹绪龙[2];宋新旺[2];崔晓红[2] [issn] => 0567-7351 [uri] => https://www.scopus.com/inward/record.uri?eid=2-s2.0-78751564648&partnerID=40&md5=39e2caaddcb270a8be1c3fdd9c7efb49 [publication_cn] => 化学学报 [title_cn] => 烷基苯磺酸盐在油水界面行为的介观模拟 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => efb04f2b4a431944a30a77d0b0b8fae4-2061735352 [hb_type] => 2 [hb_batch] => title_cn_publication_cn_pub_year_2_3 [publication_en] => ACTA CHIMICA SINICA [cite_wos] => 10 [fund_No] => 中石化重大先导试验项目(No.03003); 中石化重点项目(No.P04049)资助项目 [check_3Y] => 11 [language] => Chinese [delivery_No] => 252WW [format_title] => 1bb54e9d769bbd653e659e1e3deef2a4-563380810 [cauthor_ad] => [Li, ZQ]Shengli Oilfield, Geol Sci Res Inst, Dongying 257015, Peoples R China. [author_fn] => Li Zhen-Quan; He Xiu-Juan; Li Ying; Ma Bao-Min; Cao Xu-Long; Song Xin-Wang; Cui Xiao-Hong [reference] => Aleksey M, 2005, Phys. Chem. B, V109, P1210@@@Bresme F, 2003, J CHEM PHYS, V118, P4134, DOI 10.1063/1.1540090@@@Bresme F, 2004, LANGMUIR, V20, P5127, DOI 10.1021/la036026w@@@Conboy JC, 1998, LANGMUIR, V14, P6722, DOI 10.1021/la980132u@@@Dong FL, 2004, CHEM PHYS LETT, V399, P215, DOI@@@10.1016/j.cplett.2004.10.022@@@Groot RD, 2001, BIOPHYS J, V81, P725, DOI 10.1016/S0006-3495(01)75737-2@@@Groot RD, 1997, J CHEM PHYS, V107, P4423, DOI 10.1063/1.474784@@@HOOGERBRUGGE PJ, 1992, EUROPHYS LETT, V19, P155, DOI@@@10.1209/0295-5075/19/3/001@@@Hromadova M, 1994, J Phys Chem, V98, P11519@@@Li Y, 2005, J. Mol. Simul, V31, P1027@@@Rekvig L, 2003, LANGMUIR, V19, P8195, DOI 10.1021/la0346346@@@Richmond GL, 2002, CHEM REV, V102, P2693, DOI 10.1021/cr0006876@@@Watry MR, 2000, J AM CHEM SOC, V122, P875, DOI 10.1021/ja9917666@@@[燕永利 Yan Yongli], 2005, [化学学报, Acta Chemical Sinica], V63, P1686@@@[苑世领 YUAN ShiLing], 2006, [化学学报, Acta Chemical Sinica], V64, P1659@@@[翟利民 ZHAI LiMin], 2007, [化学学报, Acta Chemical Sinica], V65, P27 [publication_29] => ACTA CHIM SINICA [end_page] => 2808 [abstract_en] => With a simple coarse-grained model, the properties of sodium dodecylbenzene sulphonate (SDBS) adsorbed at the water/oil interface, has been investigated on a mesoscopic level by considering the variation of interfacial density using dissipative particle dynamics (DPD) simulation. Compared with sodium dodecyl sulphonate systems, sodium dodecylbenzene sulphonate are more efficient. An increase of surfactants interfacial concentration results in the increase of its interfacial density before reaching a full monolayer and appropriate salts make surfactant molecules adsorbed more at interface. It is beneficial to decrease interfacial tension if the hydrophobic chains of the surfactant and the oil have similar structure. The simulation conclusions are well consistent with the experimental results. Also with computer simulation method, we have observed that SDBS is not distributed homogeneously over the interface. Rather, the interfacial layer contains large cavities between SDBS clusters filled with water or oil clusters. When TX-100 molecules were introduced, clusters formed by nonionic surfactants filled SDBS cavities, thus decreased the interfacial tension to ultra low, even lower than 10(-3) mN.m(-1). This inhomogeneous distribution helps to enhance our understanding of the synergism interaction of the different surfactants. [author_in] => [Li, Z.-Q] Geological Scientific Research Institute, Shengli Oilfield, Dongying 257015, China@@@[ He, X.-J] Key Laboratory for Colloid and Interface Chemistry of State Education Ministry, Shandong University, Jinan 250100, China@@@[ Li, Y] Key Laboratory for Colloid and Interface Chemistry of State Education Ministry, Shandong University, Jinan 250100, China@@@[ Ma, B.-M] Key Laboratory for Colloid and Interface Chemistry of State Education Ministry, Shandong University, Jinan 250100, China@@@[ Cao, X.-L] Geological Scientific Research Institute, Shengli Oilfield, Dongying 257015, China@@@[ Song, X.-W] Geological Scientific Research Institute, Shengli Oilfield, Dongying 257015, China@@@[ Cui, X.-H] Geological Scientific Research Institute, Shengli Oilfield, Dongying 257015, China [publication_type] => J [begin_page] => 2803 [article_dt] => Article [author_en] => Li, ZQ; He, XJ; Li, Y; Ma, BM; Cao, XL; Song, XW; Cui, XH [volume] => 65 [get_data] => 2018-08-29 [publisher] => SCIENCE CHINA PRESS [keyword_en] => dissipative particle dynamics; interfacial density; interfacial; efficiency; salt alkylbenzene sulphonate [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [keyword_plu] => DISSIPATIVE PARTICLE DYNAMICS; LIQUID/LIQUID INTERFACE; SURFACTANTS; SPECTROSCOPY; EFFICIENCY [publication_iso] => Acta Chim. Sin. [format_title_en] => d7c02b8ceb0fe57916250a2314b5fec3-626384257 [publisher_city] => BEIJING [pub_date] => DEC 28 [hx_id] => 2377,2378,2371 [reference_No] => 15 [email] => yingli@sdu.edu.cn [cite_awos] => 15 [wos_No] => WOS:000252479000001 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [check_180] => 1 [publisher_ad] => 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA [title_en] => Mesoscopic simulation study on the behavior of salt alkylbenzene sulphonate adsorbed at oil/water interface [format_publication_en] => 169b60c7845c9e5f36906950b18f11111348184734 [jl_language] => chinese [jl_publication_cn] => 化学学报 [jl_article_dt] => 期刊论文 [jl_publication_en] => actachimicasinica [jl_country] => 中国,中国 [jl_keyword_en] => interfacialdensity,efficiency,saltalkylbenzenesulphonate,dissipativeparticledynamics,interfacial [jl_keyword_cn] => ,耗散颗粒动力学模拟,界面密度,界面效率,烷基苯磺酸盐 [jl_clc] => te35746 [jl_publisher] => sciencechinapress [author_id] => 21994 [author_test] => Array ( [0] => Array ( [sure] => 1 [irmagnum] => 0 [u_index] => 0 [name] => 李英 [sys_author_id] => Array ( [0] => 21994 ) [irtag] => 0 [t_index] => 0 [person_id] => 21994 ) ) [company_id] => 43,169 [sys_subject_sort] => 0,0 [college_parent_id] => 43,169 [company_test] => Array,Array [sys_author_id_arr] => [cscd_No] => CSCD:3052875 [jl_publication_cn_publication_en] => actachimicasinica,化学学报 [jl_keyword_cn_keyword_en] => 耗散颗粒动力学模拟,烷基苯磺酸盐,interfacial,interfacialdensity,saltalkylbenzenesulphonate,界面效率,efficiency,dissipativeparticledynamics,界面密度 [sys_author_id] => 21994 [format_cscd_No] => ad64b5d3187a6d7640707a2e0e67a70d-866253841 [format_title_en_publication_en_pub_year] => 25e9b125e4a375b7565ea6f322bd4b2e-569873606 [format_wos_No] => 18713130369e4fb93b0c8ca77d9e9f88-1625778125 [format_title_en_issn_pub_year] => 774530244de70fee9bf8bc482f64e3cf1774622136 [format_scopus_No] => 5d07146e4647e438f77cc7ecb61feaaa331173739 [standard_in] => Key Laboratory for Colloid and Interface Chemistry of State Education Ministry, Shandong University, Jinan 250100, China; Geological Scientific Research Institute, Shengli Oilfield, Dongying 257015, China [cauthor] => Li, Y(yingli@sdu.edu.cn) [datebase] => Scopus [page] => 2803-2808 [cite_scopus] => 11 [format_issn_issue_page_pub_year] => 7fca5629ecfab03ecee0a646008b6d66-1755253878 [sys_priority_field] => 76 [scopus_No] => 2-s2.0-78751564648 [id] => 8wozvmUBFjIhTVEbAoJx [tags] => 0 ) [19] => Array ( [batch2] => 1,2,6 [batch] => 3249,3250,3252,3254,3243,3241 [tag] => 0 [abstract_cn] => 在G3(MP2 )水平上 ,通过对CH3 S与O2 反应势能面 (PES)上关键驻点的能量计算 ,共找到 4种中间体 ,9个过渡态 ,6种产物通道 ,并对这些气相反应机理进行了讨论 ,同时应用TST RRKM理论对主要反应的速率进行计算 .结果表明 :CH3 S与O2 反应在低温下以生成CH3 SOO为主 ,并与实验结果吻合 ;在中高温下以加成消去和抽提反应为主 ,分别生成CH3 +SO2 和CH2 S +HO2 ,其它产物较少 . [keyword_cn] => 从头算方法;甲基硫自由基(CH3S);TST-RRKM理论;反应机理 [article_id] => 26626,332386,661176,581876,237805,495477 [clc] => O646 [author_jg] => [王少坤,张庆竹,曹成波,顾月姝]山东大学化学与化工学院,山东大学化学与化工学院,山东大学化学与化工学院,山东大学化学与化工学院 济南250100,济南250100,济南250100,济南250100 [format_title_cn_publication_cn_pub_year] => 6577b3c75f59c904c2719001d90e830a-1825728987 [hints] => 8 [issue] => 3 [sys_level_num] => 2_3 [sys_jg_type] => 11,5 [format_issn_issue_page_pub_year] => 82e29ec6bf9d6849babd2da0e233f4b81617301876 [source_type] => 351 [pub_year] => 2002 [pub_date] => MAR [pages] => 6 [from_id] => 76,75,73,80,85,78 [author_cn] => 王少坤,张庆竹,曹成波,顾月姝 [issn] => 0567-7351 [uri] => http://kns.cnki.net/kns/detail/detail.aspx?FileName=HXXB200203009&DbName=CJFQ2002 [publication_cn] => 化学学报 [title_cn] => CH_3S与O_2气相反应机理的理论研究 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => c1412ed7667dc8716fab5e6177883103-646764068 [page] => 432-437+379 [hb_type] => 2 [article_dt] => Article [hb_batch] => title_cn_publication_cn_pub_year_2_3 [format_title_en] => 69aac89bb01eb58c10f84fe6a8074128-1908857084 [format_title] => dd7d7e6511bd6d7e5129230c2b02868f-2141603976 [hx_id] => 2377,2378,2371 [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [format_publication_en] => 169b60c7845c9e5f36906950b18f11111348184734 [jl_publication_cn] => 化学学报 [jl_article_dt] => 期刊论文 [jl_keyword_cn] => 从头算方法,甲基硫自由基ch3s,反应机理,tstrrkm理论 [jl_clc] => o646 [author_in] => [Wang, S.-K] School of Chemistry and Chemical Industry, Shandong University, Jinan 250100, China@@@[ Zhang, Q.-Z] School of Chemistry and Chemical Industry, Shandong University, Jinan 250100, China@@@[ Cao, C.-B] School of Chemistry and Chemical Industry, Shandong University, Jinan 250100, China@@@[ Gu, Y.-S] School of Chemistry and Chemical Industry, Shandong University, Jinan 250100, China [company_id] => 0,43,169 [sys_subject_sort] => 0,0 [college_parent_id] => 43,169 [company_test] => Array,Array [author_id] => [author_test] => Array ( ) [sys_author_id_arr] => [jl_publication_cn_publication_en] => 化学学报 [jl_keyword_cn_keyword_en] => tstrrkm理论,从头算方法,反应机理,甲基硫自由基ch3s [cite_wos] => 9 [publication_en] => ACTA CHIMICA SINICA [fund_No] => 高等学校博士点专项科研基金(No. 1995042201)资助项目 [check_3Y] => 1 [language] => Chinese [delivery_No] => 533UW [cauthor_ad] => [Wang, SK]Shandong Univ, Sch Chem & Chem Ind, Jinan 250100, Peoples R China. [author_fn] => Wang, SK; Zhang, QZ; Cao, CB; Gu, YS [reference] => Baboul AG, 1999, J CHEM PHYS, V110, P7650, DOI 10.1063/1.478676@@@BALLA RJ, 1986, CHEM PHYS, V109, P101, DOI 10.1016/0301-0104(86)80188-4@@@Curtiss LA, 1999, J CHEM PHYS, V110, P4703, DOI 10.1063/1.478385@@@TURNIPSEED AA, 1992, J PHYS CHEM-US, V96, P7502, DOI 10.1021/j100198a006@@@@@@TYNDALL GS, 1991, INT J CHEM KINET, V23, P383@@@YIN FD, 1990, J ATMOS CHEM, V11, P309, DOI 10.1007/BF00053780@@@ [cite_wanfang] => 10 [cauthor] => Wang, SK(guojz@icm.sdu.edu.cn) [format_title_en_issn_pub_year] => 8aa17556a0df0d3da96cc545e96a5160939641631 [datebase] => Scopus [format_scopus_No] => 3bf16b2a057f868ddb1637bb28d03475-1913923286 [publication_29] => ACTA CHIM SINICA [end_page] => 437 [abstract_en] => A series of key stationary points of potential energy surface (PES) for the CH3S + O-2 system was calculated at the G3 (MP2) level. The calculations reveal four intermediates, nine transition states and six product channels. With the stationary points and TST-RRKM theory, the reaction rates are calculated, gas phase reaction mechanism of CH3S + O-2 is discussed. At low temperature, the reaction producing CH3SOO is the main channel. At high temperature, the addition elimination mechanism giving products of CH3 + SO2 and H-abstraction mechanism giving products of CH2S + HO2 are dominant reaction channels, the other products might be neglected. [publication_type] => J [begin_page] => 432 [author_en] => Wang, SK; Zhang, QZ; Cao, CB; Gu, YS [format_cscd_No] => 8b6e66eade8b559658ead5815c48e367-2062825452 [volume] => 60 [publisher] => SCIENCE CHINA PRESS [get_data] => 2018-08-29 [keyword_en] => ab initio; methylthiyl radical; TST-RRKM; reaction mechanism [keyword_plu] => GAUSSIAN-3 [publication_iso] => Acta Chim. Sin. [format_title_en_publication_en_pub_year] => 7f71dd92ffe19592ff6bc14edbc0348a1179263095 [cite_scopus] => 8 [publisher_city] => BEIJING [cite_cscd] => 6 [publication_info] => 0567-7351(2002)60:3<432:CYOQXF>2.0.TX;2-U [email_c] => guojz@icm.sdu.edu.cn [email] => guojz@icm.sdu.edu.cn [reference_No] => 6 [cite_awos] => 10 [cscd_No] => CSCD:1008497 [wos_No] => WOS:000174549600010 [format_wos_No] => ae11a46b84bf69652a8d47814310fcd2-1673170385 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [check_180] => 0 [publisher_ad] => 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA [standard_in] => School of Chemistry and Chemical Industry, Shandong University, Jinan 250100, China [scopus_No] => 2-s2.0-0442264869 [title_en] => Theoretical study of the gas phase reaction of CH3S with O-2 [jl_language] => chinese [jl_publication_en] => actachimicasinica [sys_author_jg_last_arr] => 济南250100 [jl_company_test] => uircu0,unameuu5316u5b66u4e0eu5316u5de5u5b66u9662,uparentidu43,uorgidu43,ulevelu1 [jl_country] => 中国 [jl_keyword_en] => tstrrkm,abinitio,reactionmechanism,methylthiylradical [sys_author_in_last_arr] => china [jl_publisher] => sciencechinapress [sys_author_id] => [id] => wQ5IvmUBFjIhTVEbRWIm [tags] => 0 ) ) 1-->
1. 钛酸铋系化合物的光催化性能研究 CSCD SCOPUS SCIE

作者:许效红;姚伟峰;张寅;周爱秋;侯云;王民

作者机构:[许效红] 山东大学,化学与化工学院, 济南, 山东 250100, 中国.;[周爱秋] 山东大学,化学与化工学院, 济南, 山东 250100, 中国.;[姚伟峰] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[张寅] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[侯云] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[王民] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2005,Vol.63,Issue.1,5-10+91

WOS被引数:20

资源类型:期刊论文

WOS:000226363200002

2. CH_3S与NO基态反应的机理及动力学 CSCD SCOPUS SCIE

作者:王少坤,张庆竹,周建华,顾月姝

作者机构:[王少坤] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[张庆竹] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[顾月姝] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[周建华] 山东轻工业学院化工系, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2004,Vol.62,Issue.6,550-555+531

WOS被引数:20

资源类型:期刊论文

WOS:000220437300004

3. 钴(Ⅱ)-丁二肟体系的吸附伏安法研究 SCIE

作者:金文睿;刘坤;

作者机构:[金文睿;刘坤]山东大学化学系,山东大学化学系 济南,济南 青岛医学院化学教研室

来源:化学学报,ACTA CHIMICA SINICA,1985,Vol.43,Issue.10,923-929

WOS被引数:19

资源类型:期刊论文

WOS:A1985AVR2900004

4. 锗烯与乙烯环加成反应的理论研究 SCOPUS SCIE

作者:卢秀慧[1];王沂轩[2]

作者机构:[卢秀慧;王沂轩;刘成卜]济南大学化学系;[卢秀慧;王沂轩;刘成卜]山东大学化学院;[卢秀慧;王沂轩;刘成卜]山东大学化学院 济南250002;[卢秀慧;王沂轩;刘成卜]济南250100;[卢秀慧;王沂轩;刘成卜]济南250100

来源:化学学报,ACTA CHIMICA SINICA,1999,Vol.57,Issue.12

WOS被引数:15

资源类型:期刊论文

WOS:000084781100010

5. 硅烯与甲醛环加成反应的理论研究 SCOPUS SCIE

作者:卢秀慧[1];王沂轩[2]

作者机构:[卢秀慧;王沂轩;刘成卜;邓从豪]济南大学化学系;[卢秀慧;王沂轩;刘成卜;邓从豪]山东大学化学院;[卢秀慧;王沂轩;刘成卜;邓从豪]山东大学化学院;[卢秀慧;王沂轩;刘成卜;邓从豪]山东大学化学院 济南250002;[卢秀慧;王沂轩;刘成卜;邓从豪]济南250100;[卢秀慧;王沂轩;刘成卜;邓从豪]济南250100;[卢秀慧;王沂轩;刘成卜;邓从豪]济南250100

来源:化学学报,ACTA CHIMICA SINICA,1998,Vol.56,Issue.11,1079-1080

WOS被引数:14

资源类型:期刊论文

WOS:000077372200006

6. 侧基含偶氮基的硅氧烷梳状聚合物的光致变色性 SCOPUS SCIE

作者:张静智;张其震

作者机构:[张静智;张其震]山东大学化学系;[张静智;张其震]山东大学化学系 济南250100;[张静智;张其震]济南250100

来源:化学学报,ACTA CHIMICA SINICA,1997,Vol.55,Issue.9,930-936

WOS被引数:14

资源类型:期刊论文

WOS:A1997YB05800016

7. 一代树状碳硅烷液晶研究—端基含12个丁氧基偶氮苯介晶基元 CSCD SCOPUS SCIE

作者:张其震[1];赵晓光[2];等

作者机构:[张其震] 山东大学化学化工学院, 济南, 山东 250100, 中国.;[刘建强] 山东大学化学化工学院, 济南, 山东 250100, 中国.;[殷晓颖] 山东大学化学化工学院, 济南, 山东 250100, 中国.;[张静智] 山东大学化学化工学院, 济南, 山东 250100, 中国.;[赵晓光] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国.;[李光] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国.;[季怡萍] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国

来源:化学学报,ACTA CHIMICA SINICA,2002,Vol.60,Issue.12,2232-2237

WOS被引数:14

资源类型:期刊论文

WOS:000179969400026

8. 亚烷基卡宾与甲醛环加成反应机理的理论研究 CSCD SCIE

作者:卢秀慧;翟利民;王沂轩;刘成卜

作者机构:[卢秀慧] 济南大学化学系, 济南, 山东 250002, 中国.;[翟利民] 济南大学化学系, 济南, 山东 250002, 中国.;[王沂轩] 山东大学化学院, 济南, 山东 250100, 中国.;[刘成卜] 山东大学化学院, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2002,Vol.60,Issue.5,769-774

WOS被引数:13

资源类型:期刊论文

WOS:000175712200003

9. 二代树状碳硅烷液晶研究Ⅰ.端基含36个丁氧基偶氮苯介晶基元 CSCD SCIE

作者:张其震,刘建强,殷晓颖,张静智,季怡萍,赵晓光,李光

作者机构:[张其震,刘建强,殷晓颖,张静智,季怡萍,赵晓光,李光]山东大学化学化工学院,山东大学化学化工学院,山东大学化学化工学院,山东大学化学化工学院,中国科学院长春应用化学研究所,中国科学院长春应用化学研究所,中国科学院长春应用化学研究所 济南250100,济南250100,济南250100,济南250100,长春130022,长春130022,长春130022

来源:化学学报,ACTA CHIMICA SINICA,2003,Vol.61,Issue.3,416-421

WOS被引数:13

资源类型:期刊论文

WOS:000182279800022

10. 邻香兰素甘氨酸三吡啶合Ni(Ⅱ)的合成、性质、晶体结构及热分解动力学 SCIE

作者:崔学桂;孙宏建;刘德信;李晓燕;李淑兰;

作者机构:[崔学桂;孙宏建;刘德信;李晓燕;李淑兰]山东大学应用化学系,山东大学应用化学系,山东大学应用化学系,山东大学应用化学系,山东大学应用化学系 济南 250100,济南 250100,济南 250100,济南 250100,济南 250100

来源:化学学报,ACTA CHIMICA SINICA,1993,Vol.51,Issue.4,346-351

WOS被引数:12

资源类型:期刊论文

WOS:A1993LF79000007

11. 石墨型C_3N_4的固态合成及嵌锂性能研究 CSCD SCOPUS SCIE

作者:杨晓晖;王红军;陆希峰;崔得良;张树永;

作者机构:[杨晓晖] 山东大学化学与化工学院, 教育部胶体与界面化学重点实验室, 济南, 山东 250100, 中国.;[王红军] 山东大学化学与化工学院, 教育部胶体与界面化学重点实验室, 济南, 山东 250100, 中国.;[张树永] 山东大学化学与化工学院, 教育部胶体与界面化学重点实验室, 济南, 山东 250100, 中国.;[陆希峰] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[崔得良] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2009,Vol.67,Issue.11,1166-1170

WOS被引数:11

资源类型:期刊论文

WOS:000267606400002

12. 三代树状碳硅烷液晶研究——端基含丁氧基偶氮苯介晶基元 CSCD SCOPUS SCIE

作者:张其震[1];殷晓颖[1];王大庆[2];李光[3];季怡萍[3];赵晓光[3]

作者机构:[张其震] 山东大学化学化工学院, 济南, 山东 201000, 中国.;[殷晓颖] 山东大学化学化工学院, 济南, 山东 201000, 中国.;[王大庆] 山东师范大学测试中心, 济南, 山东 250014, 中国.;[李光] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国.;[季怡萍] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国.;[赵晓光] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国

来源:化学学报,ACTA CHIMICA SINICA,2003,Vol.61,Issue.4,619-624

WOS被引数:11

资源类型:期刊论文

WOS:000187533500030

13. 吡啶-BH_3相互作用复合物的理论研究 CSCD SCOPUS SCIE

作者:孟凡翠,步宇翔,刘成卜

作者机构:[孟凡翠] 山东大学理论化学研究所, 济南, 山东 250100, 中国.;[刘成卜] 山东大学理论化学研究所, 济南, 山东 250100, 中国.;[步宇翔] 山东大学理论化学研究所, 分子动力学国家重点实验室, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2002,Vol.60,Issue.1,7-12+7

WOS被引数:11

资源类型:期刊论文

WOS:000173368700003

14. 混合碳链烷基聚葡糖苷中相微乳液的研究 CSCD SCOPUS SCIE

作者:柴金岭;李东祥;李干佐;梁芳珍;张高勇山东大学胶体与界面化学教育部重点实验室;夏瑞

作者机构:[柴金岭] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[李东祥] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[李干佐] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[张高勇] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[梁芳珍] 山东师范大学化学系, 济南, 山东 250014, 中国.;[夏瑞] 北京药品检验所, 北京 100035, 中国

来源:化学学报,ACTA CHIMICA SINICA,2004,Vol.62,Issue.1,47-52

WOS被引数:11

资源类型:期刊论文

WOS:000187998100010

15. 一代树状碳硅烷液晶的光化学研究——端基含12个4-丁氧基偶氮苯介晶基元 CSCD SCOPUS SCIE

作者:张其震,刘建强,殷晓颖,张静智

作者机构:[张其震,刘建强,殷晓颖,张静智]山东大学化学化工学院,山东大学化学化工学院物理与微电子学院,山东大学化学化工学院,山东大学化学化工学院 济南 250100, 济南 250100, 济南 250100, 济南 250100

来源:化学学报,ACTA CHIMICA SINICA,2003,Vol.61,Issue.7,1108-1113

WOS被引数:11

资源类型:期刊论文

WOS:000184988400026

16. 烯丙基硫脲和十二烷基硫醇对铜的缓蚀作用 CSCD SCOPUS SCIE

作者:王春涛;陈慎豪;赵世勇;李德刚

作者机构:[王春涛] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[陈慎豪] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[赵世勇] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[李德刚] 山东大学化学与化工学院, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2003,Vol.61,Issue.2,151-155

WOS被引数:10

资源类型:期刊论文

WOS:000181172200001

17. 一代树状碳硅烷液晶研究——端基含12个4-硝基偶氮苯介晶基元 CSCD SCOPUS SCIE

作者:张其震,盛昕,殷晓颖,季怡萍,李光,赵晓光

作者机构:[张其震] 山东大学化学化工学院, 济南, 山东 250100, 中国.;[盛昕] 山东大学化学化工学院, 济南, 山东 250100, 中国.;[殷晓颖] 山东大学化学化工学院, 济南, 山东 250100, 中国.;[季怡萍] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国.;[李光] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国.;[赵晓光] 中国科学院长春应用化学研究所, 长春, 吉林 130022, 中国

来源:化学学报,ACTA CHIMICA SINICA,2003,Vol.61,Issue.9,1478-1483

WOS被引数:10

资源类型:期刊论文

WOS:000188245700026

18. 含N,O和S的Schiff碱配体的双核锌配合物的合成与晶体结构 SCIE

作者:马长勤,王绪宁,张文兴,于正刚,蒋德华,董士利

作者机构:[马长勤,王绪宁,张文兴,于正刚,蒋德华,董士利]山东大学化学院,山东大学化学院,山东大学化学院,山东大学化学院,山东大学化学院,淄博市公安局 济南250100,济南250100,济南250100,济南250100,济南250100,淄博255039

来源:化学学报,ACTA CHIMICA SINICA,1996,Vol.54,Issue.6,562-567

WOS被引数:10

资源类型:期刊论文

WOS:A1996UY13200007

19. 烷基苯磺酸盐在油水界面行为的介观模拟 CSCD SCOPUS SCIE

作者:李振泉[2];何秀娟[1];李英[1];马保民[1];曹绪龙[2];宋新旺[2];崔晓红[2]

作者机构:[李振泉] 中石化胜利油田地质科学研究院, 东营, 山东 257015, 中国.;[曹绪龙] 中石化胜利油田地质科学研究院, 东营, 山东 257015, 中国.;[宋新旺] 中石化胜利油田地质科学研究院, 东营, 山东 257015, 中国.;[崔晓红] 中石化胜利油田地质科学研究院, 东营, 山东 257015, 中国.;[何秀娟] 山东大学化学与化工学院, 胶体与界面教育部重点实验室, 济南, 山东 250100, 中国.;[李英] 山东大学化学与化工学院, 胶体与界面教育部重点实验室, 济南, 山东 250100, 中国.;[马保民] 山东大学化学与化工学院, 胶体与界面教育部重点实验室, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2007,Vol.65,Issue.24,2803-2808

WOS被引数:10

资源类型:期刊论文

WOS:000252479000001

20. CH_3S与O_2气相反应机理的理论研究 CSCD SCOPUS SCIE

作者:王少坤,张庆竹,曹成波,顾月姝

作者机构:[王少坤,张庆竹,曹成波,顾月姝]山东大学化学与化工学院,山东大学化学与化工学院,山东大学化学与化工学院,山东大学化学与化工学院 济南250100,济南250100,济南250100,济南250100

来源:化学学报,ACTA CHIMICA SINICA,2002,Vol.60,Issue.3,432-437+379

WOS被引数:9

资源类型:期刊论文

WOS:000174549600010

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