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water cyclinder --> water lamellae --> continuous water phase, for this system. In the lamellae region, the dispersion exhibited negative thixotropic and shear thicken properties. The bizarre rheological properties exhibited by the dispersion with water/oil ratios of 1 were explained in terms of ion-dipole association between oleate and hexanol molecules on adjacent dropletes, which was investigated as a function of pH, ratios of water and added salts. [publication_type] => J [begin_page] => 729 [author_en] => WU, SY; CHEN, ZQ; WANG, SQ; LI, Y; YUAN, YL; ZHANG, CS [volume] => 51 [get_data] => 2018-08-29 [publisher] => ACTA CHIMICA SINICA [keyword_plu] => LIQUID-CRYSTALS; RATIO [publication_iso] => Acta Chim. Sin. [format_title_en_publication_en_pub_year] => c69b0a84942cb0221948f672b11a7a001570388038 [publisher_city] => SHANGHAI [cauthor_order] => 1 [reference_No] => 14 [cite_awos] => 5 [wos_No] => WOS:A1993LX88200001 [format_wos_No] => 33929a6ec1b2a969b71d49ec06ec876a-2044470079 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [cauthor_back] => WU, SY [check_180] => 0 [publisher_ad] => SHANGHAI INST ORGANIC CHEM ACADEMIA SINICA 345 LINGLING LU, SHANGHAI,; PEOPLES R CHINA [title_en] => THE BIZARRE RHEOLOGICAL PROPERTIES OF MICROEMULSION WITH ANIONIC SURFACTANT [sys_subject_sort] => 0,0 [college_parent_id] => 43,169 [company_test] => Array,Array [id] => 5A9KvmUBFjIhTVEbYAQa [tags] => 0 ) [17] => Array ( [batch2] => 1,2,6 [batch] => 3250,3243,3241,3252 [tag] => 0 [abstract_cn] => 合成的标题化合物晶体(C_(23)H_(29)N_3O_6Zn)属正交晶系,空间群P2_12_12_1,晶胞参数a=0.9345(2),b=2.6620(5),c=0.9748(4)nm,V=2.425(2)nm~3,Z=4利用热重分析对配合物第一步热分解过程进行了非等温动力学研究,探讨了反应的可能机理,得到其相应的动力学参数,非等温动力学方程为:da /dt=A·e~((-E)/RT)·(1—a) [keyword_cn] => Schiff碱;锌配合物;晶体结构;热分解动力学 [article_id] => 539390,170607,498964,335579 [clc] => O657.62 [author_jg] => [康永军,刘德信,李淑兰,李智红,刘亮,杨兆荷]山东省科学院,山东大学化学系,山东大学化学系,山东大学化学系,山东大学化学系,山东大学晶体材料研究所 济南250100,济南250100,济南250100,济南250100,济南250100 [format_title_cn_publication_cn_pub_year] => 9c6424d00eed1ebab1cd32489c230b731279043878 [hints] => 17 [issue] => 9 [sys_level_num] => 2_3 [sys_jg_type] => 3,5 [format_issn_issue_page_pub_year] => c8ff1dd6cb8584a7d52d2c5ed6c536d1-399122359 [source_type] => 351 [pub_year] => 1996 [pub_date] => 1996-09-20 [pages] => 7 [from_id] => 76,80,73,78 [author_cn] => 康永军,刘德信,李淑兰,李智红,刘亮,杨兆荷 [issn] => 0567-7351 [uri] => http://kns.cnki.net/kns/detail/detail.aspx?FileName=HXXB199609010&DbName=CJFQ1996 [publication_cn] => 化学学报 [title_cn] => 邻香兰素L-缬氨酸Schiff碱吡啶合锌(Ⅱ)配合物的合成、晶体结构和热分解动力学 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => c8d19d47756f30aad513885c7490de8d2016122003 [page] => 893-899 [hb_type] => 2 [article_dt] => Article [jl_publication_cn] => 化学学报 [jl_article_dt] => 期刊论文 [jl_keyword_cn] => schiff碱,锌配合物,热分解动力学,晶体结构 [jl_clc] => o65762 [author_in] => [Kang, Y.-J] Department of Chemistry, Shandong University, Jinan, 250100, China@@@[ Liu, D.-X] Department of Chemistry, Shandong University, Jinan, 250100, China@@@[ Li, S.-L] Department of Chemistry, Shandong University, Jinan, 250100, China@@@[ Li, Z.-H] Department of Chemistry, Shandong University, Jinan, 250100, China@@@[ Liu, L] Department of Chemistry, Shandong University, Jinan, 250100, China@@@[ Yang, Z.-H] Institute of Crystal Materials, Shandong University, Jinan, 250100, China [company_id] => 24,0,151,43,169 [sys_subject_sort] => 0,0,0,0 [college_parent_id] => 24,151,43,169 [company_test] => Array,Array,Array,Array [author_id] => [author_test] => Array ( ) [sys_author_id_arr] => [jl_publication_cn_publication_en] => 化学学报 [hb_batch] => grant_no [publication_en] => ACTA CHIMICA SINICA [cite_wos] => 5 [check_3Y] => 1 [language] => Japanese [delivery_No] => VN415 [format_title] => 956f6b5780adde7d7e2a4022edf44575449102919 [cauthor_ad] => [Kang, YJ]SHANDONG UNIV,DEPT CHEM,JINAN 250100,PEOPLES R CHINA. [author_fn] => Kang, YJ; Liu, DX; Li, SL; Li, ZH; Liu, L; Yang, ZH [format_title_en_issn_pub_year] => 1bbcf65cc4aa1ed345c1e5b0fa47b0b4-808858333 [datebase] => Scopus [format_scopus_No] => c31252029e256652056add4a0296e15d1666630103 [publication_29] => ACTA CHIM SINICA [end_page] => 899 [abstract_en] => The complex [Zn(L)(C5H5N)(2)]. 2H(2)O(L = 3-methoxysalicylidene-L-valine) was synthesized. The complex crystalizes in an orthorhombic system, space group is P2(1)2(1)2(1),cell parameters: a = 0.9345(2), b = 2.6620(5), c = 0.9748(4) nm, V = 2.425(2) nm(3), M(r) = 508.87, Z = 4, with R = 0.074, R(w) = 0.076. The kinetics of thermal decomposition reaction of the complex was studied under a non - isothermal condition by TG. The kinetic parameters were obtained from the analysis of TG, DTG curves by integral and differential methods. The kinetic equation of thermal decomposition reaction is:; d alpha/dt = A . e(-E/RT).(1 - alpha) [publication_type] => J [begin_page] => 893 [author_en] => Kang, YJ; Liu, DX; Li, SL; Li, ZH; Liu, L; Yang, ZH [volume] => 54 [get_data] => 2018-08-29 [publisher] => ACTA CHIMICA SINICA [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [publication_iso] => Acta Chim. Sin. [format_title_en_publication_en_pub_year] => cde1ed704bffb97f6c661e40fb9b9916642499050 [format_title_en] => 11da289eafb07fc0ead93c742e7b327e-1640036457 [publisher_city] => SHANGHAI [cauthor_order] => 1 [hx_id] => 2378,2371 [reference_No] => 5 [cite_awos] => 5 [wos_No] => WOS:A1996VN41500011 [format_wos_No] => 38dac908c5116307c38e0880eb880377-569701572 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [cauthor_back] => Kang, YJ [check_180] => 0 [publisher_ad] => SHANGHAI INST ORGANIC CHEM ACADEMIA SINICA 345 LINGLING LU, SHANGHAI,; PEOPLES R CHINA [standard_in] => Department of Chemistry, Shandong University, Jinan, 250100, China; Institute of Crystal Materials, Shandong University, Jinan, 250100, China [scopus_No] => 2-s2.0-33750134395 [title_en] => Synthesis, crystal structure and kinetics of thermal decomposition of the complex of o-vanillin-L-valine-dipyridine zinc(II) [format_publication_en] => 169b60c7845c9e5f36906950b18f11111348184734 [jl_language] => japanese [jl_publication_en] => actachimicasinica [sys_author_jg_last_arr] => 济南250100 [jl_company_test] => uircu0,uorgidu24,uparentidu24,unameuu6676u4f53u6750u6599u7814u7a76u6240,ulevelu1 [jl_country] => 中国 [sys_author_in_last_arr] => china [jl_publisher] => actachimicasinica [sys_author_id] => [id] => 6g9KvmUBFjIhTVEbYAQa [tags] => 0 ) [18] => Array ( [batch2] => 1,2,6 [batch] => 3249,3250,3241,3254,3243,3252 [tag] => 0 [abstract_cn] => 合成了一种新的导电分子晶体(PyH)[Ni(dmit)2]2(Py=pyridine,dmit=(C3S5)2-=4,5-dimercapto-1,3-dithiole-2-thione),用元素分析、红外光谱对其进行了表征,并用四圆X射线衍射方法确定了结构,该晶体属于三斜晶系,P-1空间群;晶胞参数为:a=0.59227(4)nm,b=0.82279(6)nm,c=1.67535(9)nm,α=90.233(5)°,β=92.107(5)°,y=104.654(6)°;V=0.78925(9)nm3,Z=1.(PyH)[Ni(dnit)2]2晶体中,导电组元[Ni(dmit)2]-0.5沿b轴方向形成具有二聚体结构的柱状堆积,在(001)面形成以肩并肩分子间的S…S强相互作用为特征的二维导电层,这种二维导电层上的室温电导率为0.13 Ω-1@cm-1,在c轴方向,(PyH)+与[Ni(dmit)2]-0.5之间除库仑作用外,还存在N-H…S,C-H…S氢键相互作用.单晶(001)面上变温电阻的测定结果表明,在∞K到室温的温度范围内,(PyH)[Ni-(dmit)2]2具有半导体导电行为,导电激活能为0.15eV. [keyword_cn] => 分子导体;合成;结构;导电性;(PyH)[Ni(dmit)2]2;镍配合物;吡啶阳离子; [clc] => O614.813 O62 [author_jg] => [许文] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.@@@[方奇] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.@@@[薛刚] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.@@@[于文涛] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.@@@[刘国群] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.@@@[张德清] 中国科学院化学研究所, 北京 100080, 中国.@@@[徐伟] 中国科学院化学研究所, 北京 100080, 中国.@@@[徐翠英] 中国科学院化学研究所, 北京 100080, 中国.@@@[张金彪] 中国科学院化学研究所, 北京 100080, 中国 [format_title_cn_publication_cn_pub_year] => 6499107f99c3d181905973520d25e76d1492037491 [from_id] => 76,75,73,80,78,85 [issue] => 12 [sys_level_num] => 2_1 [sys_jg_type] => 10,2,5 [source_type] => 351 [pub_year] => 2002 [article_id] => 664457,597876,239542,495072,331653,82202 [pages] => 6 [hints] => 16 [author_cn] => 许文[1];方奇[1];薛刚[1];于文涛[1];刘国群[1];张德清[2];徐伟[2];徐翠英[2];张金彪[2] [issn] => 0567-7351 [uri] => https://www.scopus.com/inward/record.uri?eid=2-s2.0-0442267256&partnerID=40&md5=4bc35a1e51fb54cd313530f3ddd13316 [publication_cn] => 化学学报 [title_cn] => 分子导体(PyH)[Ni(dmit)2]2的合成、结构与导电性 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => 061d7847c3e6b582f7e1b5738c863adf-186056764 [hb_type] => 2 [hb_batch] => title_cn_publication_cn_pub_year_2_3 [publication_en] => ACTA CHIMICA SINICA [cite_wos] => 5 [fund_No] => 国家自然科学基金(Nos.20172034 and 29672023); 中国科学院有机固体开放实验室资助项目 [check_3Y] => 3 [language] => Chinese [delivery_No] => 628AK [format_title] => ec1357904dbe01adea3bf1c6673912ef-1302797810 [cauthor_ad] => [Xu, W]Shandong Univ, State Key Lab Crystal Mat, Jinan 250100, Peoples R China. [author_fn] => Xu, W; Fang, Q; Xue, G; Yu, WT; Liu, GQ; Zhang, DQ; Xu, W; Xu, CY; Zhang, JB [reference] => BOUSSEAU M, 1986, J AM CHEM SOC, V108, P1908, DOI 10.1021/ja00268a032@@@BROSSARD L, 1989, J PHYS-PARIS, V50, P1521, DOI@@@10.1051/jphys:0198900500120152100@@@Fang Q, 2002, J CHEM SOC DALTON, P1377, DOI 10.1039/b105854c@@@KOBAYASHI A, 1987, CHEM LETT, P1819, DOI 10.1246/cl.1987.1819@@@KOBAYASHI A, 1991, CHEM LETT, P2163, DOI 10.1246/cl.1991.2163@@@KOBAYASHI H, 1992, CHEM LETT, P1909, DOI 10.1246/cl.1992.1909@@@MIYAZAKI A, 1992, B CHEM SOC JPN, V65, P2528, DOI 10.1246/bcsj.65.2528@@@@@@STEIMECKE G, 1979, PHOSPHORUS SULFUR, V7, P49, DOI@@@10.1080/03086647808069922@@@@@@TAJIMA H, 1993, CHEM LETT, P1235, DOI 10.1246/cl.1993.1235@@@Veldhuizen YSJ, 1997, INORG CHEM, V36, P4930, DOI 10.1021/ic970347b@@@@@@Xu W, 2001, SYNTHETIC MET, V122, P409, DOI 10.1016/S0379-6779(00)00405-7 [publication_29] => ACTA CHIM SINICA [end_page] => 2158 [abstract_en] => A new molecular conductor ( PyH) [ Ni ( dmit)(2)](2) ( Py = pyridine, dmit = ( C3S5)(2-) = 4,5-dimercapto-1,3-dithiole-2-thione) has been prepared by oxidation with I-2/NaI and characterized by elemental analysis and IR spectrum. The single crystal structure was determined by four-circle X-ray diffraction method. Crystallographic parameters for (PyH) [Ni(dmit)(2)](2): triclinic system; P-1 space group; a = 0.59227 (4) nm, b =0.82279(6) mn, c = 1.67535(9) nm, alpha = 90.233(5)degrees, beta = 92.107(6)degrees, gamma = 104.654(6)degrees; V = 0. 78925 (9) nm; Z = 1. Both [Ni (dmit)(2)](-0.5) anion and PyH+ cation are almost planar. [Ni(dmit)(2)](-0.5) is stacked to form columns of dimerised pairs along the b-axis. Short and intense (SS)-S-... contacts in side-by-side style build a kind of two-dimensional network in the (001) plane. The conductivity at one direction on (001) plane at room temperature was measured to be 0.13 Omega(-1) (.) cm(-1). Along the c direction the sheets of conductive [Ni(dTnit)(2)](-0.5) are structurally modulated by hydrogen bonds between anions and cations. The resistivity-temperature curve in the temperature range of 90 - 290 K shows that the title compound behaves as a semiconductor with quite narrow energy gap. [orcID] => Liu, Guoqun/0000-0002-3342-5780 [author_in] => [Xu, W] State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China@@@[ Fang, Q] State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China@@@[ Xue, G] State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China@@@[ Yu, W.-T] State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China@@@[ Liu, G.-Q] State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China@@@[ Zhang, D.-Q] Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080, China@@@[ Xu, W] Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080, China@@@[ Xu, C.-Y] Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080, China@@@[ Zhang, J.-B] Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080, China [publication_type] => J [begin_page] => 2153 [article_dt] => Article [author_en] => Xu, W; Fang, Q; Xue, G; Yu, WT; Liu, GQ; Zhang, DQ; Xu, W; Xu, CY; Zhang, JB [volume] => 60 [get_data] => 2018-08-29 [publisher] => SCIENCE CHINA PRESS [keyword_en] => molecular conductor; synthesis; structure; electrical conductivity [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [keyword_plu] => CRYSTAL-STRUCTURE; SUPERCONDUCTOR; TRANSITION; METAL [publication_iso] => Acta Chim. Sin. [format_title_en] => a11f3e9d635d7fcdcbb9497005493383274661362 [publisher_city] => BEIJING [pub_date] => DEC [hx_id] => 2377,2378,2371 [reference_No] => 11 [email] => Fangqi@icm.sdu.edu.cn [cite_awos] => 6 [wos_No] => WOS:000179969400013 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [check_180] => 0 [publisher_ad] => 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA [title_en] => Synthesis, structure and conductivity of molecular conductor (PyH)[Ni(dmit)(2)](2) [format_publication_en] => 169b60c7845c9e5f36906950b18f11111348184734 [jl_language] => chinese [jl_publication_cn] => 化学学报 [jl_article_dt] => 期刊论文 [jl_publication_en] => actachimicasinica [jl_country] => 中国,中国 [jl_keyword_en] => electricalconductivity,synthesis,structure,molecularconductor [jl_keyword_cn] => 镍配合物,pyhnidmit22,,结构,分子导体,吡啶阳离子,导电性,合成 [jl_clc] => o614813o62 [jl_publisher] => sciencechinapress [company_id] => 24,151 [sys_subject_sort] => 0,0 [college_parent_id] => 24,151 [company_test] => Array,Array [author_id] => 24843,20672,25191 [author_test] => Array ( [0] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 0 [name] => 方奇 [irtag] => 7 [t_index] => 0 [person_id] => 20672 ) [1] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 0 [name] => 许文 [irtag] => 7 [t_index] => 0 [person_id] => 24843 ) [2] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 0 [name] => 于文涛 [irtag] => 7 [t_index] => 0 [person_id] => 25191 ) ) [sys_author_id_arr] => 20672方奇 [cscd_No] => CSCD:1139004 [jl_publication_cn_publication_en] => actachimicasinica,化学学报 [jl_keyword_cn_keyword_en] => pyhnidmit22,导电性,吡啶阳离子,合成,镍配合物,electricalconductivity,分子导体,synthesis,molecularconductor,structure,结构 [sys_author_id] => 20672 [format_cscd_No] => 54a27f1ce147c97201828ed1e6dd6032-24558549 [format_title_en_publication_en_pub_year] => e6f6e780a542e84ac9438cfa8cd2321a826992157 [format_wos_No] => a740437d3e5efa467c8392f29643bddf426507591 [format_title_en_issn_pub_year] => 7042a0234f6175b35dd542ca120ac50b390139824 [format_scopus_No] => 325b1794eda6a234c7f3a3d205d2d0e1693878080 [standard_in] => State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China; Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080, China [datebase] => Scopus [page] => 2153-2158 [cite_scopus] => 5 [format_issn_issue_page_pub_year] => 0d02885845544868f2344810f6807e0e1673518242 [sys_priority_field] => 76 [scopus_No] => 2-s2.0-0442267256 [id] => KAkwvmUBFjIhTVEbmrnE [tags] => 0 ) [19] => Array ( [batch2] => 1,2,6 [uri] => https://www.scopus.com/inward/record.uri?eid=2-s2.0-84877682408&doi=10.6023%2fA13010068&partnerID=40&md5=fc94e2a0a3e148646ebbe2fce0f17074 [tag] => 0 [abstract_cn] => 采用分子动力学方法研究了吸附在聚二甲基硅氧烷(PDMS)和接枝聚磺酸基甜菜碱甲基丙烯酸甲酯(pSBMA)改性后的防污材料膜水化层内的水分子的结构及其动力学性质,从微观角度解释了聚合物膜具有防污性能的原因.模拟发现:(1)紧靠聚合物膜形成的水化层是聚合物具有防污性能的关键因素,该水化层是溶液中的粒子(包括蛋白质分子)与聚合物膜相接触时所要克服的最主要的物理能障;(2)相对PDMS聚合物膜而言,双离子特性自组装膜(pSBMA)在氢键、静电力的共同作用下,可以形成空间笼状水分子网结构对水分子具有更强的束缚作用并有效降低水分子的可运动性,形成的稳定水化层使得pSBMA具有更强的阻碍蛋白质吸附的能力. [keyword_cn] => 聚二甲基硅氧烷;;聚磺酸基甜菜碱甲基丙烯酸甲酯;;生物污损;;防污材料;;分子动力学 [fund_No] => Science and Technology on Marine Corrosion and Protection Laboratory; Open Research Fund [KF120404]; National Natural Science Foundation of; China [21173128] [article_id] => 368386,455009,59797,660512,155322,534848 [clc] => O657.3 [author_jg] => [张恒] 山东大学化学与化工学院, 海洋腐蚀与防护国家级重点实验室, 济南, 山东 250100, 中国.@@@[王华] 山东大学化学与化工学院, 济南, 山东 250100, 中国.@@@[苑世领] 山东大学化学与化工学院, 济南, 山东 250100, 中国.@@@[蔺存国] 中国船舶重工集团公司第七二五研究所, 海洋腐蚀与防护国家级重点实验室, 青岛, 山东 266101, 中国.@@@[王利] 中国船舶重工集团公司第七二五研究所, 海洋腐蚀与防护国家级重点实验室, 青岛, 山东 266101, 中国 [format_title_cn_publication_cn_pub_year] => cda560e51397f9022fd44e45516cfaf9-1846393101 [hints] => 58 [issue] => 4 [author_first] => 张恒; [sys_level_num] => 2_3 [sys_jg_type] => 11,3,5 [format_issn_issue_page_pub_year] => e2076206e6e1764d0252acfb076940c81570611315 [source_type] => 351 [pub_year] => 2013 [pub_date] => APR 15 [pages] => 8 [from_id] => 76,75,73,80,78,85 [author_cn] => 张恒;王华;蔺存国;王利;苑世领; [issn] => 0567-7351 [batch] => 3249,3250,3252,3254,3243,3241 [publication_cn] => 化学学报 [title_cn] => 聚合物防污材料表面水化层的分子动力学模拟 [CSSN] => 31-1320/O6 [SYS_TAG] => 3 [format_title_cn_issn_pub_year] => 15e0b96ec0d53dcff94356c78ee8854b-263996279 [page] => 649-656 [hb_type] => 2 [article_dt] => Article [hb_batch] => title_cn_publication_cn_pub_year_2_3 [cite_wos] => 5 [publication_en] => ACTA CHIMICA SINICA [check_3Y] => 65 [language] => Chinese [delivery_No] => 135AQ [format_title] => ee1aeea2180da04aa5f5f2bc9031c1a52001299975 [cauthor_ad] => [Zhang, H]Shandong Univ, Sch Chem & Chem Engn, Jinan 250100, Peoples R China. [author_fn] => Zhang Heng; Wang Hua; Lin Cunguo; Wang Li; Yuan Shiling [reference] => Accelrys Software Inc, 2008, Materials Studio, Release 4.4@@@AHMED EI, 2009, MACROMOLECULES, V42, P3186@@@Andrea M., 2012, J MOL MODEL, V18, P239@@@Berendsen H. J. C., 1981, INTERMOLECULAR FORCE, V14, P331@@@Besseling NAM, 1997, LANGMUIR, V13, P2113, DOI 10.1021/la960672w@@@Chen H, 2008, MACROMOL BIOSCI, V8, P863, DOI 10.1002/mabi.200800014@@@Chen SF, 2005, J AM CHEM SOC, V127, P14473, DOI 10.1021/ja054169u@@@Chen SF, 2006, LANGMUIR, V22, P8186, DOI 10.1021/la061012m@@@Cheng G, 2007, BIOMATERIALS, V28, P4192, DOI@@@10.1016/j.biomaterials.2007.05.041@@@Gaberc P. V., 2008, CURR OPIN DRUG DISC, V11, P242@@@[何腾云 He Tengyun], 2007, [涂料工业, Paint & coatings industry], V37, P59@@@He Y, 2008, PHYS CHEM CHEM PHYS, V10, P5539, DOI 10.1039/b807129b@@@He Y, 2008, LANGMUIR, V24, P10358, DOI 10.1021/la8013046@@@Hess B, 2008, J. Chem. Theory Comput, V4, P425@@@Hower JC, 2006, J CHEM PHYS, V125, DOI 10.1063/1.2397681@@@Hower J C, 2006, J CHEM PHYS, V125@@@Ladd J, 2008, BIOMACROMOLECULES, V9, P1357, DOI 10.1021/bm701301s@@@Laredo J, 2004, J VASC SURG, V39, P1059, DOI 10.1016/j.jvs.2003.12.025@@@Morra M, 2000, J BIOMAT SCI-POLYM E, V11, P547, DOI@@@10.1163/156856200743869@@@Ostuni E, 2001, LANGMUIR, V17, P5605, DOI 10.1021/la010384m@@@Schuler LD, 2001, J COMPUT CHEM, V22, P1205, DOI 10.1002/jcc.1078@@@Shao Q, 2010, J PHYS CHEM B, V114, P16625, DOI 10.1021/jp107272n@@@[史航 Shi Hang], 2009, [涂料工业, Paint & Coatings Industry], V39, P10@@@Teare DOH, 2005, J PHYS CHEM B, V109, P20923, DOI 10.1021/jp052767p@@@Vaisocherova H, 2008, ANAL CHEM, V80, P7894, DOI 10.1021/ac8015888@@@VAN DER SPOEL D, 2005, J COMPUT CHEM, V26, P1701@@@Vanderah DJ, 2004, J AM CHEM SOC, V126, P13639, DOI 10.1021/ja047744n@@@Yang W, 2008, LANGMUIR, V24, P9211, DOI 10.1021/la801487f@@@Yang W, 2009, BIOMATERIALS, V30, P5617, DOI@@@10.1016/j.biomaterials.2009.06.036@@@Zhang Z, 2006, J PHYS CHEM B, V110, P10799, DOI 10.1021/jp057266i@@@Zhang Z, 2008, BIOMATERIALS, V29, P4285, DOI@@@10.1016/j.biomaterials.2008.07.039@@@Zhang Z, 2006, LANGMUIR, V22, P10072, DOI 10.1021/la062175d@@@Zheng J, 2004, LANGMUIR, V20, P8931, DOI 10.1021/la036345n@@@Zheng J, 2005, BIOPHYS J, V89, P158, DOI 10.1529/biophysj.105.059428 [open_type] => gold_or_bronze [publication_29] => ACTA CHIM SINICA [end_page] => 656 [abstract_en] => The prevention of nonspecific protein adsorption was a big challenge in biomedical and marine fields. Recent studies of the mechanisms of non-fouling materials have identified a strong correlation between material surface hydration and resistance to nonspecific protein adsorption. To investigate the molecular mechanism of two typical non-fouling materials PDMS and pSBMA on molecular level, a series of molecular dynamics simulations were conducted. This work concentrated on the structure properties and dynamic behaviors of water molecules that belong to the non-fouling membranes\' surface hydration layers. Water\'s behavior near the membrane were analyzed in energetic, dynamics and structure aspects: PMFs (potential of mean force) between hydration layer water and polymer surfaces indicated pSBMA has more advantages on binding water molecules energetically; the analyzing of diffusion coefficients, residence time, and dipole residence time of hydration layer water showed pSBMA has slower dynamics properties which demonstrate water molecules were tightly bonded by pSBMA; the illustration of atoms density profile, hydrogen bond and their number distribution showed a rich hydrogen bond network structure around pSBMA. Based on above, following conclusions were then speculated: 1) the hydration layer near non-fouling membrane has a strong relationship with the nonspecific protein adsorption which forms a physical and energy barrier during particles in solution (including proteins) come into contact with non-fouling membranes. 2) Comparing with PDMS, pSBMA as a zwitterionic polymer can bind water molecules more strongly via both electrostatic and hydrogen bonding. And the caging effects of water network formed around pSBMA can also reduce water molecules\' mobility. All these lead to a stable hydration layer that prevents non-specific protein adsorption. Simply, pSBMA generated a more energetic advantaged, tightly bounded and structured water layer by electrostatic, hydrogen bonding and caging effect. This hydration layer prevents protein from approaching the surface, resulting in a better non-fouling surface than PDMS. [author_in] => [Zhang, H] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China, Science and Technology on Marine Corrosion and Protection Laboratory, Luoyang Ship Material Research Institute (LSMRI), Qingdao 266101, China@@@[ Wang, H] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China@@@[ Lin, C] Science and Technology on Marine Corrosion and Protection Laboratory, Luoyang Ship Material Research Institute (LSMRI), Qingdao 266101, China@@@[ Wang, L] Science and Technology on Marine Corrosion and Protection Laboratory, Luoyang Ship Material Research Institute (LSMRI), Qingdao 266101, China@@@[ Yuan, S] School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China [publication_type] => J [begin_page] => 649 [author_en] => Zhang, H; Wang, H; Lin, CG; Wang, L; Yuan, SL [volume] => 71 [get_data] => 2018-08-29 [publisher] => SCIENCE PRESS [keyword_en] => poly-dimethylsiloxane; poly-sulfobetaine methacrylate; bio-fouling;; non-fouling material; molecular dynamics [format_publication_cn] => 6918be3b26b1fa6ec0424f6071208a75331227575 [keyword_plu] => SELF-ASSEMBLED MONOLAYERS; PROTEIN ADSORPTION; STRONG RESISTANCE; SULFOBETAINE; PLASMA; WATER; CARBOXYBETAINE; FORCES; SERUM [doi] => 10.6023/A13010068 [publication_iso] => Acta Chim. Sin. [fund_ab] => Project supported by the Science and Technology on Marine Corrosion and; Protection Laboratory Open Research Fund (No. KF120404) and the National; Natural Science Foundation of China (No. 21173128). [format_title_en] => 0e86c4f86574965bc96266e6136e14c5-283804489 [publisher_city] => BEIJING [hx_id] => 2377,2378,2371 [reference_No] => 33 [email] => shilingyuan@sdu.edu.cn [cite_awos] => 5 [wos_No] => WOS:000318258800026 [wos_sub] => Chemistry, Multidisciplinary [research_area] => Chemistry [check_180] => 2 [publisher_ad] => 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA [title_en] => Molecular Dynamics Simulations of Surface Hydration Layers Near Non-fouling Polymer Membranes [format_publication_en] => 169b60c7845c9e5f36906950b18f11111348184734 [jl_language] => chinese [jl_publication_cn] => 化学学报 [jl_article_dt] => 期刊论文 [jl_publication_en] => actachimicasinica [jl_country] => 中国,中国 [jl_keyword_en] => ,moleculardynamics,polydimethylsiloxane,biofouling,polysulfobetainemethacrylate,nonfoulingmaterial [jl_keyword_cn] => ,聚磺酸基甜菜碱甲基丙烯酸甲酯,聚二甲基硅氧烷,生物污损,分子动力学,防污材料 [jl_clc] => o6573 [jl_publisher] => sciencepress [author_id] => 25263,25411 [author_test] => Array ( [0] => Array ( [sure] => 0 [irmagnum] => 0 [u_index] => 5 [name] => 苑世领 [irtag] => 9 [t_index] => 0 [person_id] => 25263 ) [1] => Array ( [sure] => 1 [irmagnum] => 0 [u_index] => 1 [name] => 张恒 [sys_author_id] => Array ( [0] => 25411 ) [irtag] => 0 [t_index] => 0 [person_id] => 25411 ) ) [company_id] => 0,43,169 [sys_subject_sort] => 0,0 [college_parent_id] => 43,169 [company_test] => Array,Array [sys_author_id_arr] => 25411张恒 [cscd_No] => CSCD:4812055 [jl_publication_cn_publication_en] => actachimicasinica,化学学报 [jl_keyword_cn_keyword_en] => polysulfobetainemethacrylate,防污材料,moleculardynamics,polydimethylsiloxane,生物污损,biofouling,分子动力学,聚二甲基硅氧烷,nonfoulingmaterial,聚磺酸基甜菜碱甲基丙烯酸甲酯 [sys_author_id] => 25263,25411 [format_cscd_No] => 72d81b143ed8bf7ba3f1d341375ed021739191542 [format_title_en_publication_en_pub_year] => 13e9bc1af439d04a33fb12b68cdf2721-1806728867 [format_wos_No] => d1385c3d5d520d41be87892306d68be01947154200 [format_title_en_issn_pub_year] => 4964a7409f8d66beee80ba1d66726157277572869 [format_scopus_No] => 7dab61e78c20a7583a81887b86bc9f0e521282764 [standard_in] => School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, China; Science and Technology on Marine Corrosion and Protection Laboratory, Luoyang Ship Material Research Institute (LSMRI), Qingdao 266101, China [cauthor] => Yuan, S(shilingyuan@sdu.edu.cn) [datebase] => Scopus [cite_scopus] => 7 [sys_priority_field] => 76 [scopus_No] => 2-s2.0-84877682408 [id] => _g9KvmUBFjIhTVEbryH8 [tags] => 0 ) ) 1-->
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68. 丙烯酸聚乙二醇酯-甲基丙烯酸共聚物对CaCO_3微粒形貌的调控 CSCD SCOPUS SCIE

作者:王芳,徐桂英,张志庆,肖莉

作者机构:[王芳] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[徐桂英] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[张志庆] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[肖莉] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2003,Vol.61,Issue.9,1488-1491

WOS被引数:5

资源类型:期刊论文

WOS:000188245700028

69. Mg-Al-NO_3层状双金属氢氧化物电性质研究 CSCD SCOPUS SCIE

作者:金志琳,侯万国,张春光,孙祉伟,杨亲正,孙德军,戴国亮

作者机构:[金志林] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[侯万国] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[张春光] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[孙祉伟] 中国科学院力学研究所, 国家微重力实验室, 北京 100080, 中国

来源:化学学报,ACTA CHIMICA SINICA,2003,Vol.61,Issue.8,1208-1212

WOS被引数:5

资源类型:期刊论文

WOS:000185643800009

70. 用环糊精合成楔筒状主体分子新模型 CSCD SCIE

作者:郝爱友;王金山

作者机构:[郝爱友] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[王金山] 山东师范大学化学系, 济南, 山东 250014, 中国

来源:化学学报,ACTA CHIMICA SINICA,2002,Vol.60,Issue.8,1536-1538+1356

WOS被引数:5

资源类型:期刊论文

WOS:000177641800033

71. 液铜快速冷却过程微观结构演变的计算机模拟 CSCD SCOPUS SCIE

作者:张弢;吴爱玲;管立;齐元华;徐昌业

作者机构:[张弢] 山东大学物理与微电子学院, 济南, 山东 250061, 中国.;[管立] 山东大学物理与微电子学院, 济南, 山东 250061, 中国.;[齐元华] 山东大学物理与微电子学院, 济南, 山东 250061, 中国.;[徐昌业] 山东大学物理与微电子学院, 济南, 山东 250061, 中国.;[吴爱玲] 山东大学物理与微电子学院, 济南, 山东 25006, 中国

来源:化学学报,ACTA CHIMICA SINICA,2003,Vol.61,Issue.9,1357-1361

WOS被引数:5

资源类型:期刊论文

WOS:000188245700004

72. 二硝酸二(N-月桂酰吡咯烷)合铀酰配合物的合成和结构 SCOPUS SCIE

作者:韩景田,包伯荣,孙国新,杨勇,杨永会,陈民勤,孙思修

作者机构:[韩景田,包伯荣,孙国新,杨勇,杨永会,陈民勤,孙思修]中国科学院上海原子核研究所,上海大学理学院,中国科学院上海原子核研究所,复旦大学分析测试中心,山东大学化学学院,复旦大学分析测试中心,山东大学化学学院 上海201800,上海201800,上海201800,上海200433,济南250100,上海200433,济南250100

来源:化学学报,ACTA CHIMICA SINICA,2000,Vol.58,Issue.10,1286-1290

WOS被引数:5

资源类型:期刊论文

WOS:000165207800021

73. 硼氮掺杂的碳纳米管对硫化氢气敏性能的理论研究 CSCD SCOPUS SCIE

作者:王若曦;张冬菊;武剑;刘成卜;

作者机构:[王若曦] 山东大学理论化学研究所, 济南, 山东 250100, 中国.;[张冬菊] 山东大学理论化学研究所, 济南, 山东 250100, 中国.;[武剑] 山东大学理论化学研究所, 济南, 山东 250100, 中国.;[刘成卜] 山东大学理论化学研究所, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2007,Vol.65,Issue.2,107-110

WOS被引数:5

资源类型:期刊论文

WOS:000244172300004

74. Zn-Al类水滑石零净电荷点及等电点研究 CSCD SCOPUS SCIE

作者:李丽芳,侯万国,戴肖南,刘春霞

作者机构:[李丽芳] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[侯万国] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[戴肖南] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[刘春霞] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2004,Vol.62,Issue.4,429-432+343

WOS被引数:5

资源类型:期刊论文

WOS:000189108900017

75. 一代碳硅烷树枝状大分子钯配合物的液晶性 CSCD SCOPUS SCIE

作者:张其震;殷晓颖;李爱香;王艳

作者机构:[张其震] 山东大学化学化工学院,中国.;[殷晓颖] 山东大学化学化工学院,中国.;[杨爱香] 山东大学化学化工学院,中国.;[王艳] 山东大学环境与工程学院, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2005,Vol.63,Issue.10,934-940+871

WOS被引数:5

资源类型:期刊论文

WOS:000229327000012

76. 漆酶在纳米多孔金上的固定化及其酶学性质研究 CSCD SCOPUS SCIE

作者:邱华军[1];徐彩霞[1];姬广磊[1];黄锡荣[1,2];韩书华[1];丁轶[1];曲音波[2]

作者机构:[邱华军] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[徐彩霞] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[姬广磊] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[黄锡荣] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[韩书华] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[丁轶] 山东大学, 胶体与界面化学教育部重点实验室, 济南, 山东 250100, 中国.;[曲音波] 山东大学, 微生物技术国家重点实验室, 济南, 山东 250100, 中国

来源:化学学报,ACTA CHIMICA SINICA,2008,Vol.66,Issue.18,2075-2080

WOS被引数:5

资源类型:期刊论文

WOS:000259904300010

77. 阴离子型表面活性剂所组成微乳液的异常流变性 SCIE

作者:伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜;

作者机构:[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]青岛化工学院应用化学系;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]青岛化工学院应用化学系;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]青岛化工学院应用化学系;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]青岛化工学院应用化学系;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]山东大学化学系;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]山东大学化学系 青岛 266042;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]青岛 266042;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]青岛 266042;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]青岛 266042;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]济南 250100;[伍世英;陈宗淇;王世权;李莹;袁云龙;张传胜]济南 250100

来源:化学学报,ACTA CHIMICA SINICA,1993,Vol.51,Issue.8,729-735

WOS被引数:5

资源类型:期刊论文

WOS:A1993LX88200001

78. 邻香兰素L-缬氨酸Schiff碱吡啶合锌(Ⅱ)配合物的合成、晶体结构和热分解动力学 SCOPUS SCIE

作者:康永军,刘德信,李淑兰,李智红,刘亮,杨兆荷

作者机构:[康永军,刘德信,李淑兰,李智红,刘亮,杨兆荷]山东省科学院,山东大学化学系,山东大学化学系,山东大学化学系,山东大学化学系,山东大学晶体材料研究所 济南250100,济南250100,济南250100,济南250100,济南250100

来源:化学学报,ACTA CHIMICA SINICA,1996,Vol.54,Issue.9,893-899

WOS被引数:5

资源类型:期刊论文

WOS:A1996VN41500011

79. 分子导体(PyH)[Ni(dmit)2]2的合成、结构与导电性 CSCD SCOPUS SCIE

作者:许文[1];方奇[1];薛刚[1];于文涛[1];刘国群[1];张德清[2];徐伟[2];徐翠英[2];张金彪[2]

作者机构:[许文] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[方奇] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[薛刚] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[于文涛] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[刘国群] 山东大学, 晶体材料国家重点实验室, 济南, 山东 250100, 中国.;[张德清] 中国科学院化学研究所, 北京 100080, 中国.;[徐伟] 中国科学院化学研究所, 北京 100080, 中国.;[徐翠英] 中国科学院化学研究所, 北京 100080, 中国.;[张金彪] 中国科学院化学研究所, 北京 100080, 中国

来源:化学学报,ACTA CHIMICA SINICA,2002,Vol.60,Issue.12,2153-2158

WOS被引数:5

资源类型:期刊论文

WOS:000179969400013

80. 聚合物防污材料表面水化层的分子动力学模拟 CSCD SCOPUS SCIE

作者:张恒;王华;蔺存国;王利;苑世领;

作者机构:[张恒] 山东大学化学与化工学院, 海洋腐蚀与防护国家级重点实验室, 济南, 山东 250100, 中国.;[王华] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[苑世领] 山东大学化学与化工学院, 济南, 山东 250100, 中国.;[蔺存国] 中国船舶重工集团公司第七二五研究所, 海洋腐蚀与防护国家级重点实验室, 青岛, 山东 266101, 中国.;[王利] 中国船舶重工集团公司第七二五研究所, 海洋腐蚀与防护国家级重点实验室, 青岛, 山东 266101, 中国

来源:化学学报,ACTA CHIMICA SINICA,2013,Vol.71,Issue.4,649-656

WOS被引数:5

资源类型:期刊论文

WOS:000318258800026

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